Pyromellitic Diimides: Minimal Cores for High Mobility n-Channel Transistor Semiconductors

被引：114

作者：

Zheng, Qingdong

Huang, Jia

Sarjeant, Amy

Katz, Howard E. ^{[1
]}

机构：

[1] Johns Hopkins Univ, Dept Mat Sci & Engn, Baltimore, MD 21218 USA

来源：

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY | 2008年 / 130卷 / 44期

关键词：

D O I：

10.1021/ja805746h

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Three pyromellitic diimides were synthesized in high yields by one conventional reaction between pyromellitic dianhydride and various amines. The films made from these pyromellitic diimides derivatives exhibit a mobility up to 0.079 cm(2)/(V.s). In addition, the on/off ratios of n-channel devices are as high as 1 000 000.

引用

收藏

页码：14410 / +

页数：3

相关论文

共 22 条

[1] Functionalized acenes and heteroacenes for organic electronics [J].

Anthony, John E. .

CHEMICAL REVIEWS, 2006, 106 (12) :5028-5048

[2] Tetrathiafulvalenes, oligoacenenes, and their buckminsterfullerene derivatives: The brick and mortar of organic electronics [J].

Bendikov, M ;

Wudl, F ;

Perepichka, DF .

CHEMICAL REVIEWS, 2004, 104 (11) :4891-4945

[3] Redox modulation of benzene triimides and diimides via noncovalent interactions [J].

Carroll, JB ;

Gray, M ;

McMenimen, KA ;

Hamilton, DG ;

Rotello, VM .

ORGANIC LETTERS, 2003, 5 (18) :3177-3180

[4] Air stable n-channel organic semiconductors for thin film transistors based on fluorinated derivatives of perylene diimides [J].

Chen, H. Z. ;

Ling, M. M. ;

Mo, X. ;

Shi, M. M. ;

Wang, M. ;

Bao, Z. .

CHEMISTRY OF MATERIALS, 2007, 19 (04) :816-824

[5] Large-scale complementary integrated circuits based on organic transistors [J].

Crone, B ;

Dodabalapur, A ;

Lin, YY ;

Filas, RW ;

Bao, Z ;

LaDuca, A ;

Sarpeshkar, R ;

Katz, HE ;

Li, W .

NATURE, 2000, 403 (6769) :521-523

[6] Dibenzotetrathiafulvalene bisimides: New building blocks for organic electronic materials [J].

Gao, Xike ;

Wang, Ying ;

Yang, Xiaodi ;

Liu, Yunqi ;

Qiu, Wenfeng ;

Wu, Weiping ;

Zhang, Hengjun ;

Qi, Ting ;

Liu, Ying ;

Lu, Kun ;

Du, Chunyan ;

Shuai, Zhigang ;

Yu, Gui ;

Zhu, Daoben .

ADVANCED MATERIALS, 2007, 19 (19) :3037-+

[7] Reduction in operation voltage of complementary organic thin-film transistor inverter circuits using double-gate structures [J].

Hizu, Kazuki ;

Sekitani, Tsuyoshi ;

Someya, Takao ;

Otsuki, Joe .

APPLIED PHYSICS LETTERS, 2007, 90 (09)

[8] Hydroxy-terminated organic semiconductor-based field-effect transistors for phosphonate vapor detection [J].

Huang, Jia ;

Miragliotta, Joseph ;

Becknell, Alan ;

Katz, Howard E. .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2007, 129 (30) :9366-9376

[9] High-mobility air-stable n-type semiconductors with processing versatility:: Dicyanoperylene-3,4:9,10-bis(dicarboximides) [J].

Jones, BA ;

Ahrens, MJ ;

Yoon, MH ;

Facchetti, A ;

Marks, TJ ;

Wasielewski, MR .

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2004, 43 (46) :6363-6366

[10] Tuning orbital energetics in arylene diimide semiconductors. Materials design for ambient stability of n-type charge transport [J].

Jones, Brooks A. ;

Facchetti, Antonio ;

Wasielewski, Michael R. ;

Marks, Tobin J. .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2007, 129 (49) :15259-15278