Seasonal variation of aerosol composition at Cheju Island, Korea

被引:108
作者
Carmichael, GR
Zhang, Y
Chen, LL
Hong, MS
Ueda, H
机构
[1] UNIV IOWA,DEPT CHEM & BIOCHEM ENGN,IOWA CITY,IA 52242
[2] AJOU UNIV,DEPT ENVIRONM ENGN,SEOUL,SOUTH KOREA
[3] KYUSHU UNIV,DEPT APPL MECH,FUKUOKA 812,JAPAN
关键词
aerosols; enrichment factors; dust; aerosol modeling;
D O I
10.1016/1352-2310(95)00230-8
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A preliminary assessment of the seasonal variation in chemical composition of aerosols measured at Cheju Island, Korea, is presented. Weekly and monthly averaged aerosol composition derived from 15 months of daily filter measurements are presented. The annual-average non-sea-salt sulfate and nitrate mass concentrations of aerosols measured at Cheju are found to be 6.9 mu g m(-3) and 1.2 mu g m(-3), respectively; calcium and potassium are present in nearly equal quantities at similar to 0.5 mu g m(-3), and ammonium averaged 1.4 mu g m(-3). Each species is found to follow a seasonal cycle with sulfate, nitrate, ammonium, potassium and calcium all showing up to 50% higher values in the spring. In contrast, chlorine is 30% lower in the spring. Aerosol enrichment factors relative to the composition of seawater and crustal material from the Gobi dust-source region in China are also presented. The aerosol measured at Cheju is found to be enriched in sulfate, nitrate and ammonium, but deficient in chlorine (relative to seawater). These results along with modeling studies suggest that the dust surfaces play an important role in nitrate and sulfate formation. Copyright (C) 1996 Elsevier Science Ltd
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页码:2407 / 2416
页数:10
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