Sulfur and Nitrogen Dual-Doped Mesoporous Graphene Electrocatalyst for Oxygen Reduction with Synergistically Enhanced Performance

被引:1993
作者
Liang, Ji [1 ]
Jiao, Yan [1 ]
Jaroniec, Mietek [2 ]
Qiao, Shi Zhang [1 ]
机构
[1] Univ Adelaide, Sch Chem Engn, Adelaide, SA 5005, Australia
[2] Kent State Univ, Dept Chem & Biochem, Kent, OH 44242 USA
基金
澳大利亚研究理事会;
关键词
graphene; heterogeneous catalysis; nanostructures; oxygen reduction reaction; synergistic effects; METAL-FREE ELECTROCATALYSTS; NANOSHEETS; NANOTUBES; CATALYST; ARRAYS; BORON;
D O I
10.1002/anie.201206720
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Doping duo: Mesoporous graphene doped with both N and S atoms (N-S-G) was prepared in one step and studied as an electrochemical catalyst for the oxygen reduction reaction (ORR). The catalyst shows excellent ORR performance comparable to that of commercial Pt/C. The outstanding activity of N-S-G results from both the large number and the synergistic effect of the dopant heteroatoms. Copyright © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
引用
收藏
页码:11496 / 11500
页数:5
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