Dynamic Spin Ice: Pr2Sn2O7

被引:96
作者
Zhou, H. D. [1 ,2 ]
Wiebe, C. R. [1 ,2 ]
Janik, J. A. [1 ,2 ]
Balicas, L. [2 ]
Yo, Y. J. [2 ]
Qiu, Y. [3 ,4 ]
Copley, J. R. D. [3 ]
Gardner, J. S. [3 ,5 ]
机构
[1] Florida State Univ, Dept Phys, Tallahassee, FL 32306 USA
[2] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32306 USA
[3] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA
[4] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA
[5] Indiana Univ, Bloomington, IN 47408 USA
关键词
D O I
10.1103/PhysRevLett.101.227204
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
In this Letter, we report a new spin ice-Pr(2)Sn(2)O(7)-which appears to have enhanced residual entropy due to the dynamic nature of the spins. Neutron scattering experiments show that at 200 mK, there is a significant amount of magnetic diffuse scattering which can be fit to the dipolar spin-ice model. However, these short-ranged ordered spins have a quasielastic response that is atypical of the canonical spin ices, and suggests that the ground state is dynamic (i.e., composed of locally ordered two-in-two-out spin configurations that can tunnel between energetically equivalent orientations). We report this as an example of a dynamic spin ice down to 200 mK.
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页数:4
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