Depth, radiocarbon, and the effectiveness of direct CO2 injection as an ocean carbon sequestration strategy -: art. no. 1766

被引:17
作者
Caldeira, K
Wickett, ME
Duffy, PB
机构
[1] Lawrence Livermore Natl Lab, Climate & Carbon Cycle Modeling Grp, Livermore, CA 94550 USA
[2] Lawrence Livermore Natl Lab, Ctr Appl Sci Comp, Livermore, CA 94550 USA
关键词
D O I
10.1029/2001GL014234
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
[1] If radiocarbon were a good predictor of the amount of time until a water parcel returns to the surface, it could be used to estimate the effectiveness of carbon sequestration by direct injection. We performed direct CO2 injection simulations in both one-dimensional box-diffusion and three-dimensional ocean general circulation models. The 1-D model results for ocean carbon retention accord with the 3-D model results, especially in the Pacific basin and at shallower depths. In the 1-D model, carbon retention in the ocean is directly related to both the injection depth and the Delta(14)C of carbon at the injection location. However, in the 3-D model, depth, but not radiocarbon, provides a relatively good prediction of carbon retention. This suggests that the expected time for a water parcel to return to the surface is closely related to its depth and not in general to the time since last at the surface.
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