Two-pulse laser control of nuclear and electronic motion

被引：10

作者：

Gronager, M

Henriksen, NE

机构：

[1] Department of Chemistry, Technical University of Denmark, DTU 207

来源：

CHEMICAL PHYSICS LETTERS | 1997年 / 278卷 / 1-3期

关键词：

D O I：

10.1016/S0009-2614(97)00967-6

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

We discuss an explicitly time-dependent two-pulse laser scheme for controlling where nuclei and electrons are going in unimolecular reactions. We focus on electronic motion and show, with HD+ as an example, that one can find non-stationary states where the electron (with some probability) oscillates back and forth between the two nuclei. We discuss how this finding can be used in a scheme for controlling electron transfer in real-time. (C) 1997 Elsevier Science B.V.

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页码：166 / 174

页数：9

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