Atmospheric emissions of F, As, Se, Hg, and Sb from coal-fired power and heat generation in China

被引:130
作者
Chen, Jian [1 ,2 ]
Liu, Guijian [1 ,2 ]
Kang, Yu [1 ]
Wu, Bin [1 ]
Sun, Ruoyu [1 ]
Zhou, Chuncai [1 ]
Wu, Dun [1 ]
机构
[1] Univ Sci & Technol China, Sch Earth & Space Sci, CAS Key Lab Crust Mantle Mat & Environm, Hefei 230026, Anhui, Peoples R China
[2] Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian 710075, Shaanxi, Peoples R China
基金
中国国家自然科学基金;
关键词
Atmospheric emissions; Toxic trace elements; Coal-fired power and heat generation; China; ANTHROPOGENIC MERCURY EMISSIONS; TRACE-ELEMENTS; ENVIRONMENTAL GEOCHEMISTRY; COMBUSTION RESIDUES; MINING DISTRICT; HEALTH IMPACTS; PLANTS; FLUORINE; SPECIATION; GUIZHOU;
D O I
10.1016/j.chemosphere.2012.10.032
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Coal is one of the major energy resources in China, with nearly half of produced Chinese coal used for power and heat generation. The large use of coal for power and heat generation in China may result in significant atmospheric emissions of toxic volatile trace elements (i.e. F, As, Se, Hg, and Sb). For the purpose of estimating the atmospheric emissions from coal-fired power and heat generation in China, a simple method based on coal consumption, concentration and emission factor of trace element was adopted to calculate the gaseous emissions of elements F, As, Se, Hg, and Sb. Results indicate that about 162161, 236, 637, 172, and 33 t F, As, Se, Hg, and Sb, respectively, were introduced into atmosphere from coal combustion by power and heat generation in China in 2009. The atmospheric emissions of F, As, Se, Hg, and Sb by power and heat generation increased from 2005 to 2009 with increasing coal consumptions. Crown Copyright (C) 2012 Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:1925 / 1932
页数:8
相关论文
共 121 条
[1]   Environmental impact of a coal combustion-desulphurisation plant:: Abatement capacity of desulphurisation process and environmental characterisation of combustion by-products [J].
Alvarez-Ayuso, E. ;
Querol, X. ;
Tomas, A. .
CHEMOSPHERE, 2006, 65 (11) :2009-2017
[2]  
Andren A.W., 1975, Environmental Science and Technology, V9, P856, DOI DOI 10.1021/ES60107A002
[3]  
[Anonymous], CHIN J CONTROL ENDEM
[4]  
[Anonymous], 2006, GEOLOGICAL STUDY CLE
[5]  
[Anonymous], 2019, Global Mercury Assessment 2018
[6]  
[Anonymous], 2002, COAL GEOL CHINA
[7]  
[Anonymous], 1998, COAL GEOL EXPLOR
[8]  
[Anonymous], COAL SCI TECHNOLOGY
[9]  
Bai X., 2007, Coal Qual. Technol, V1, P1, DOI [10.1016/j.coal.2011.02.003, DOI 10.1016/J.COAL.2011.02.003]
[10]  
Chen J, 2007, ELECT POWER ENV PROT, V23, P45