Geochronological studies of the eastern Otago Schist and adjacent metagreywacke sequences are applied to their structural/metamorphic history and schist protoliths. Rb-Sr whole-rock isochron and K-Ar total-rock ages are inversely correlated with metamorphic grade (both in terms of mineral facies and textural zones), dating the time of peak metamorphism and/or postmetamorphic cooling. On the northern flank of the schists, older ages (200-230 Ma) date initial burial metamorphism and deformation in late Triassic - early Jurassic times. Younger age patterns (to 115 Ma) reflect either (1) higher grade metamorphism during a single event followed by long-continued uplift, or (2) early burial metamorphism at >200 Ma with a second, regional metamorphism between then and 115 Ma followed by rapid uplift. Initial Sr isotopic ratios derived from isochrons indicate that protoliths originate in two terranes. North of Dunedin, initial Sr-87/Sr-86 ratios range from 0.7064 to 0.7092, similar to Torlesse Terrane (Rakaia Subterrane) analogues in the Wellington region, and indicate a granitoid source dominated by I-types. South of Dunedin, along the south Otago coast, schists have lower initial Sr-87/Sr-86 ratios, 0.7052 to 0.7064, unlike Caples-type rocks elsewhere in Otago. They are thus of ''uncertain'' terrane affinity but indicate a dominantly silicic-intermediate volcanic source.