Xe adsorption and separation properties of a series of microporous metal-organic frameworks (MOFs) with V-shaped linkers

被引：44

作者：

Banerjee, Debasis ^{[1
]}

Elsaidi, Sameh K. ^{[1
,2
]}

Thallapally, Praveen K. ^{[1
]}

机构：

[1] Pacific Northwest Natl Lab, Phys & Computat Sci Directorate, Richland, WA 99352 USA

[2] Alexandria Univ, Fac Sci, Dept Chem, POB 426, Alexandria 21321, Egypt

来源：

JOURNAL OF MATERIALS CHEMISTRY A | 2017年 / 5卷 / 32期

关键词：

NOBLE-GAS ADSORPTION; COMMENSURATE ADSORPTION; XENON ADSORPTION; STABILITY; CAPTURE; KRYPTON; CALCIUM; DESIGN; LIGAND; ENERGY;

D O I：

10.1039/c7ta02746j

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

A series of microporous metal-organic frameworks (MOFs) constructed by using a V-shaped linker, 4,40-sulfonyldibenzoic acid, were evaluated for their Xe gas adsorption properties. In particular, a cadmium-based MOF exhibits noteworthy Xe adsorption and separation properties in the presence of other gases under nuclear reprocessing conditions. The outstanding Xe adsorption capacity was attributed to the close pore size matching of the MOF with the kinetic diameter of the Xe atom.

引用

页码：16611 / 16615

页数：5

共 51 条

[1]

[Anonymous], 2013, STATE BIRDS 2013 REP, P1

[2]

[Anonymous], 2013, Inventory of US greenhouse gas emissions and sinks: 1990-2011, P1

[3]

[Anonymous], 2012, BLUE RIBB COMM AM EN

[4] Direct structural evidence of commensurate-to-incommensurate transition of hydrocarbon adsorption in a microporous metal organic framework [J].

Banerjee, Debasis ;

Wang, Hao ;

Gong, Qihan ;

Plonka, Anna M. ;

Jagiello, Jacek ;

Wu, Haohan ;

Woerner, William R. ;

Emge, Thomas J. ;

Olson, David H. ;

Parise, John B. ;

Li, Jing .

CHEMICAL SCIENCE, 2016, 7 (01) :759-765

[5] Metal-organic framework with optimally selective xenon adsorption and separation [J].

Banerjee, Debasis ;

Simon, Cory M. ;

Plonka, Anna M. ;

Motkuri, Radha K. ;

Liu, Jian ;

Chen, Xianyin ;

Smit, Berend ;

Parise, John B. ;

Haranczyk, Maciej ;

Thallapally, Praveen K. .

NATURE COMMUNICATIONS, 2016, 7

[6] Potential of Metal-Organic Frameworks for Separation of Xenon and Krypton [J].

Banerjee, Debasis ;

Cairns, Amy J. ;

Liu, Jian ;

Motkuri, Radha K. ;

Nune, Satish K. ;

Fernandez, Carlos A. ;

Krishna, Rajamani ;

Strachan, Denis M. ;

Thallapally, Praveen K. .

ACCOUNTS OF CHEMICAL RESEARCH, 2015, 48 (02) :211-219

[7] Adsorption equilibria of O2, Ar, Kr and Xe on activated carbon and zeolites: single component and mixture data [J].

Bazan, R. E. ;

Bastos-Neto, M. ;

Moeller, A. ;

Dreisbach, F. ;

Staudt, R. .

ADSORPTION-JOURNAL OF THE INTERNATIONAL ADSORPTION SOCIETY, 2011, 17 (02) :371-383

[8] A metal-organic framework-based splitter for separating propylene from propane [J].

Cadiau, A. ;

Adil, K. ;

Bhatt, P. M. ;

Belmabkhout, Y. ;

Eddaoudi, M. .

SCIENCE, 2016, 353 (6295) :137-140

[9]

Chen L, 2014, NAT MATER, V13, P954, DOI [10.1038/nmat4035, 10.1038/NMAT4035]

[10] Direct Observation of Xe and Kr Adsorption in a Xe-Selective Microporous Metal-Organic Framework [J].

Chen, Xianyin ;

Plonka, Anna M. ;

Banerjee, Debasis ;

Krishna, Rajamani ;

Schaef, Herbert T. ;

Ghose, Sanjit ;

Thallapally, Praveen K. ;

Parise, John B. .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2015, 137 (22) :7007-7010

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