Electrode and Catalyst Durability Requirements in Automotive PEM Applications: Technology Status of a Recent MEA Design and Next Generation Challenges

被引:10
作者
Haas, H. R. [1 ]
Davis, M. T. [1 ]
机构
[1] Automot Fuel Cell Cooperat, Burnaby, BC V5J 5J8, Canada
来源
PROTON EXCHANGE MEMBRANE FUEL CELLS 9 | 2009年 / 25卷 / 01期
关键词
STABILITY;
D O I
10.1149/1.3210718
中图分类号
O646 [电化学、电解、磁化学];
学科分类号
081704 ;
摘要
The functionality of fuel cell vehicles is continuously being improved by several automakers and efforts are being made to demonstrate performance, durability, efficiency and freeze start capability comparable to conventional vehicles. Recent results demonstrating acceptable operational performance, efficiency, freeze start capability and durability are shown and discussed. The main barrier preventing fuel cells from being competitive with conventional ICE is the high cost of the stack and system. For the stack, the key cost driver is catalyst loading. Requirements for future catalysts are presented, demonstrating the challenges and technology gaps following from a reduction of catalyst loadings as well as the use of Pt/Co based catalysts.
引用
收藏
页码:1623 / 1631
页数:9
相关论文
共 9 条
[1]   The stability of Pt-M (M = first row transition metal) alloy catalysts and its effect on the activity in low temperature fuel cells - A literature review and tests on a Pt-Co catalyst [J].
Antolini, Ermete ;
Salgado, Jose R. C. ;
Gonzalez, Ernesto R. .
JOURNAL OF POWER SOURCES, 2006, 160 (02) :957-968
[2]   Stability of platinum based alloy cathode catalysts in PEM fuel cells [J].
Colón-Mercado, HR ;
Popov, BN .
JOURNAL OF POWER SOURCES, 2006, 155 (02) :253-263
[3]   Kinetic model of platinum dissolution in PEMFCs [J].
Darling, RM ;
Meyers, JP .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2003, 150 (11) :A1523-A1527
[4]   Activity of ordered and disordered Pt-Co alloy phases for the electroreduction of oxygen in catalysts with multiple coexisting phases [J].
Koh, Shirlaine ;
Yu, Chengfel ;
Mani, Prasanna ;
Srivastava, Ratndeep ;
Strasser, Peter .
JOURNAL OF POWER SOURCES, 2007, 172 (01) :50-56
[5]  
Ntravitsky T. Ripenbein, 2006, J POWER SOURCES, V161, P782
[6]   A reverse-current decay mechanism for fuel cells [J].
Reiser, CA ;
Bregoli, L ;
Patterson, TW ;
Yi, JS ;
Yang, JDL ;
Perry, ML ;
Jarvi, TD .
ELECTROCHEMICAL AND SOLID STATE LETTERS, 2005, 8 (06) :A273-A276
[7]   Pt-Co/C electrocatalysts for oxygen reduction in H2/O2 PEMFCs synthesized by borohydride method [J].
Salgado, JRC ;
Antolini, E ;
Gonzalez, ER .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2004, 151 (12) :A2143-A2149
[8]   PtCo/C cathode catalyst for improved durability in PEMFCs [J].
Yu, P ;
Pemberton, M ;
Plasse, P .
JOURNAL OF POWER SOURCES, 2005, 144 (01) :11-20
[9]   Evaluation of the stability and durability of Pt and Pt-Co/C catalysts for polymer electrolyte membrane fuel cells [J].
Zignani, Sabrina C. ;
Antolini, Ermete ;
Gonzalez, Ernesto R. .
JOURNAL OF POWER SOURCES, 2008, 182 (01) :83-90