Cluster formation by direct laser vaporization: evidence for the twofold mechanism

被引:22
作者
Liu, XH [1 ]
Zhang, XG [1 ]
Li, Y [1 ]
Wang, XY [1 ]
Lou, NQ [1 ]
机构
[1] Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
基金
中国国家自然科学基金;
关键词
D O I
10.1016/S0009-2614(98)00360-1
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 [物理化学]; 081704 [应用化学];
摘要
In this Letter we report experimental evidence relevant to the mechanism of cluster formation by direct laser vaporization of chemical compounds. The mechanism is different due to the type of samples and the type of clusters produced. While the clusters are formed generally through gas-phase recombination reactions, some clusters possess similar stoichiometry to the precursor sample, which, together with the velocity distribution, suggests a direct surface ejection mechanism. (C) 1998 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:804 / 808
页数:5
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