First zipper-featured molecular duplexes driven by cooperative donor-acceptor interaction

被引:62
作者
Zhou, QZ
Jiang, XK
Shao, XB
Chen, GJ
Jia, MX
Li, ZT
机构
[1] Chinese Acad Sci, Shanghai Inst Organ Chem, Shanghai 200032, Peoples R China
[2] Beijing Normal Univ, Dept Chem, Beijing 100875, Peoples R China
关键词
D O I
10.1021/ol034549p
中图分类号
O62 [有机化学];
学科分类号
070303 ; 081704 ;
摘要
[GRAPHIC] The first class of zipper-shaped artificial duplexes, which are driven by multiple donor-acceptor interactions between electron-rich 1,5-dioxynaphthalene or 1,4-dioxybenzene and electron-deficient pyromellitic dimide units, have been studied in organic media by H-1 NMR, UV-vis, and vapor pressure osmometry. H-1 NMR binding investigations reveal substantial cooperativity of the donor-acceptor interaction in the duplexes.
引用
收藏
页码:1955 / 1958
页数:4
相关论文
共 41 条
[1]   OLYMPIADANE [J].
AMABILINO, DB ;
ASHTON, PR ;
REDER, AS ;
SPENCER, N ;
STODDART, JF .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION IN ENGLISH, 1994, 33 (12) :1286-1290
[2]   Building molecular wires from the colours of life: conjugated porphyrin oligomers [J].
Anderson, HL .
CHEMICAL COMMUNICATIONS, 1999, (23) :2323-2330
[3]   THE SELF-ASSEMBLY OF A HIGHLY ORDERED [2]CATENANE [J].
ASHTON, PR ;
BROWN, CL ;
CHRYSTAL, EJT ;
GOODNOW, TT ;
KAIFER, AE ;
PARRY, KP ;
PHILP, D ;
SLAWIN, AMZ ;
SPENCER, N ;
STODDART, JF ;
WILLIAMS, DJ .
JOURNAL OF THE CHEMICAL SOCIETY-CHEMICAL COMMUNICATIONS, 1991, (09) :634-639
[4]   Strong dimerization of ureidopyrimidones via quadruple hydrogen bonding [J].
Beijer, FH ;
Sijbesma, RP ;
Kooijman, H ;
Spek, AL ;
Meijer, EW .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1998, 120 (27) :6761-6769
[5]  
BERDAGUE P, 1993, B SOC CHIM FR, V130, P475
[6]  
Berl V, 2001, CHEM-EUR J, V7, P2810, DOI 10.1002/1521-3765(20010702)7:13<2810::AID-CHEM2810>3.0.CO
[7]  
2-5
[8]   Synthesis and recognition properties of aromatic amide oligomers: Molecular zippers [J].
Bisson, AP ;
Carver, FJ ;
Eggleston, DS ;
Haltiwanger, RC ;
Hunter, CA ;
Livingstone, DL ;
McCabe, JF ;
Rotger, C ;
Rowan, AE .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2000, 122 (37) :8856-8868
[9]  
Carver FJ, 2001, CHEM-EUR J, V7, P4854, DOI 10.1002/1521-3765(20011119)7:22<4854::AID-CHEM4854>3.3.CO
[10]  
2-R