Bulk morphology and diameter distribution of single-walled carbon nanotubes synthesized by catalytic decomposition of hydrocarbons

被引:287
作者
Cheng, HM
Li, F
Sun, X
Brown, SDM
Pimenta, MA
Marucci, A
Dresselhaus, G
Dresselhaus, MS
机构
[1] Acad Sinica, Inst Met Res, Shenyang 110015, Peoples R China
[2] MIT, Dept Phys, Cambridge, MA 02139 USA
[3] MIT, Francis Bitter Natl Magnet Lab, Cambridge, MA 02139 USA
[4] MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA
基金
中国国家自然科学基金; 美国国家科学基金会;
关键词
D O I
10.1016/S0009-2614(98)00479-5
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Long and wide ropes/ribbons of single-walled carbon nanotube (SWNT) bundles with rope diameters of 100 mu m and lengths to 3 cm were synthesized by the catalytic decomposition of hydrocarbons. These ropes/ribbons consist of roughly-aligned bundles of aligned SWNTs. The SWNT diameters, as determined from HRTEM images, are 1.69 +/- 0.34 nm, which, in combination with resonant Raman scattering measurements, indicates that our SWNTs have larger diameters than those synthesized by other techniques. The larger SWNTs are promising for gas-storage applications. The easy manipulation of the ropes offer special opportunities for their characterization and applications. (C) 1998 Published by Elsevier Science B.V. All rights reserved.
引用
收藏
页码:602 / 610
页数:9
相关论文
共 23 条
  • [1] Nanometre-size tubes of carbon
    Ajayan, PM
    Ebbesen, TW
    [J]. REPORTS ON PROGRESS IN PHYSICS, 1997, 60 (10) : 1025 - 1062
  • [2] BANDOW S, 1998, IN PRESS PHYS REV LE
  • [3] Single-electron transport in ropes of carbon nanotubes
    Bockrath, M
    Cobden, DH
    McEuen, PL
    Chopra, NG
    Zettl, A
    Thess, A
    Smalley, RE
    [J]. SCIENCE, 1997, 275 (5308) : 1922 - 1925
  • [4] BROWN SDM, 1998, MRS S P BOST, V496
  • [5] CHENG HM, 1998, IN PRESS APPL PHYS L, V72
  • [6] Elastic properties of single-walled carbon nanotubes in compression
    Cornwell, CF
    Wille, LT
    [J]. SOLID STATE COMMUNICATIONS, 1997, 101 (08) : 555 - 558
  • [7] Storage of hydrogen in single-walled carbon nanotubes
    Dillon, AC
    Jones, KM
    Bekkedahl, TA
    Kiang, CH
    Bethune, DS
    Heben, MJ
    [J]. NATURE, 1997, 386 (6623) : 377 - 379
  • [8] Nanotechnology - New tricks with nanotubes
    Dresselhaus, MS
    [J]. NATURE, 1998, 391 (6662) : 19 - 20
  • [9] DRESSELHAUS MS, 1996, SCI FULLENES CARBON
  • [10] DRESSELHAUS MS, 1997, UNPUB SPECIAL LECT C