Surface modification of low cost carbons for their application in the environmental protection

被引:136
作者
Arenillas, A [1 ]
Rubiera, F [1 ]
Parra, JB [1 ]
Ania, CO [1 ]
Pis, JJ [1 ]
机构
[1] CSIC, Inst Nacl Carbon, E-33080 Oviedo, Spain
关键词
CO2; capture; carbon materials; plastic waste; adsorption;
D O I
10.1016/j.apsusc.2005.02.076
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
In this work, the CO2 capture capacity of a series of activated carbons derived froth recycled polyethylene terephtalate (PET) was tested, facing two problems at the same time: minimising plastic waste and developing an adsorbent for CO2 capture. The PET raw material, obtained from post-consumer soft-drink bottles, was chemically activated with KOH. In addition, a series of nitrogen-enriched activated carbons was obtained by mixing the raw material with different nitrogen compounds (i.e., acridine, carbazole and urea). The influence of temperature on the CO2 capture capacity of the adsorbents was evaluated in a thermogravimetric system. The CO2 uptake was also related to the chemical and textural charactefistics of the samples. (c) 2005 Elsevier B.V. All rights reserved.
引用
收藏
页码:619 / 624
页数:6
相关论文
共 18 条
[1]   Adsorption/oxidation of hydrogen sulfide on nitrogen-containing activated carbons [J].
Adib, F ;
Bagreev, A ;
Bandosz, TJ .
LANGMUIR, 2000, 16 (04) :1980-1986
[2]  
*ASS PLAST MAN EUR, 2001, AN PLAST CONS REC W
[3]   Bituminous coal-based activated carbons modified with nitrogen as adsorbents of hydrogen sulfide [J].
Bagreev, A ;
Menendez, JA ;
Dukhno, I ;
Tarasenko, Y ;
Bandosz, TJ .
CARBON, 2004, 42 (03) :469-476
[4]   Study of pyrolysis and incineration of disposable plastics using combined TG/FT-IR technique [J].
Bhandare, PS ;
Lee, BK ;
Krishnan, K .
JOURNAL OF THERMAL ANALYSIS, 1997, 49 (01) :361-366
[5]   SOME ASPECTS OF THE SURFACE-CHEMISTRY OF CARBON-BLACKS AND OTHER CARBONS [J].
BOEHM, HP .
CARBON, 1994, 32 (05) :759-769
[6]  
BOEHM HP, 1966, ADV CATAL, P1
[7]   Water adsorption on activated carbons with different degrees of oxidation [J].
CarrascoMarin, F ;
Mueden, A ;
Centeno, TA ;
Stoeckli, F ;
MorenoCastilla, C .
JOURNAL OF THE CHEMICAL SOCIETY-FARADAY TRANSACTIONS, 1997, 93 (12) :2211-2215
[8]  
Derbyshire F., 2001, CHEM PHYS CARBON
[9]  
DUNININ MM, 1975, PROG SURF MEMBR SCI, V9, P10
[10]   Removal of SOx and NOx over activated carbon fibers [J].
Mochida, I ;
Korai, Y ;
Shirahama, M ;
Kawano, S ;
Hada, T ;
Seo, Y ;
Yoshikawa, M ;
Yasutake, A .
CARBON, 2000, 38 (02) :227-239