A new thermophoretic precipitator for collection of nanometer-sized aerosol particles

被引:50
作者
Gonzalez, D
Nasibulin, AG
Baklanov, AM
Shandakov, SD
Brown, DP
Queipo, P
Kauppinen, EI
机构
[1] VTT Proc, Aerosol Technol Grp, FIN-02044 Espoo, Finland
[2] Helsinki Univ Technol, Dept Engn Phys & Math, FIN-02150 Espoo, Finland
[3] Helsinki Univ Technol, Ctr New Mat, FIN-02150 Espoo, Finland
[4] Russian Acad Sci, Inst Chem Kinet & Combust, Siberian Branch, Novosibirsk 630090, Russia
[5] Kemerovo State Univ, Gen Phys Dept, Kemerovo 650043, Russia
基金
芬兰科学院; 俄罗斯基础研究基金会;
关键词
D O I
10.1080/02786820500385569
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
A new thermophoretic precipitator (TP) has been designed and used for the collection of nanosized aerosol particles. NaCl and Fe particles, with mean diameters of 55 nm and 3.6 nm, respectively, were used to determine the thermophoretic deposition efficiency as well as the uniformity of the deposition. When the average temperature gradients applied were 2200 K/cm and 2400 K/cm, a high thermophoretic deposition efficiency, close to 100%, was attained at aerosol flow rates below 15 sccm. A gradual decay in the efficiency was observed as the flow rate was increased. Theoretical calculations of particle deposition efficiency were in good agreement with experimental data. The deposition along the TP was shown to be homogenous on a millimeter scale for both NaCl and Fe particles collected on thin foil substrates and microscope grids, respectively. Finally, the thermophoretic precipitator was used to efficiently deposit Fe nanoparticles on a substrate for the subsequent growth of carbon nanotubes.
引用
收藏
页码:1064 / 1071
页数:8
相关论文
共 29 条
[1]  
Babichev A. P., 1991, FIZICHESKIE VELICHIN
[2]   Utilization of selected area electron diffraction patterns for characterization of air submicron particulate matter collected by a thermophoretic precipitator [J].
Bang, JJ ;
Trillo, EA ;
Murr, LE .
JOURNAL OF THE AIR & WASTE MANAGEMENT ASSOCIATION, 2003, 53 (02) :227-236
[3]   THEORY OF THERMAL FORCES ACTING ON AEROSOL PARTICLES [J].
BROCK, JR .
JOURNAL OF COLLOID SCIENCE, 1962, 17 (08) :768-&
[4]  
BROWN DP, 1994, P 1994 INT JOINT POW, P69
[5]  
BROWN DP, 2005, UNPUB COMPUTERS FLUI
[6]   ELECTROSPRAY IONIZATION FOR MASS-SPECTROMETRY OF LARGE BIOMOLECULES [J].
FENN, JB ;
MANN, M ;
MENG, CK ;
WONG, SF ;
WHITEHOUSE, CM .
SCIENCE, 1989, 246 (4926) :64-71
[7]   Molecular and nanoscale materials and devices in electronics [J].
Fu, L ;
Cao, LC ;
Liu, YQ ;
Zhu, DB .
ADVANCES IN COLLOID AND INTERFACE SCIENCE, 2004, 111 (03) :133-157
[8]  
Fuchs N.A., 1964, MECH AEROSOLS
[9]   Mechanisms of electrospray ionization of singly and multiply charged salt clusters [J].
Gamero-Castaño, M ;
de la Mora, JF .
ANALYTICA CHIMICA ACTA, 2000, 406 (01) :67-91
[10]  
Green H. L., 1935, PHYS METHODS ESTIMAT