Crossover from XY critical to tricritical behavior of heat capacity at the smectic-A-chiral-smectic-C liquid-crystal transition

被引:32
作者
Ema, K [1 ]
Yao, H [1 ]
机构
[1] Tokyo Inst Technol, Fac Sci, Dept Phys, Meguro Ku, Tokyo 152, Japan
关键词
D O I
10.1103/PhysRevE.57.6677
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
High-resolution ac calorimetric measurements have been carried out for four chiral liquid-crystal systems: 4-(1-methylheptyloxycarbonyl) phenyl 4'-octyloxybiphenyl-4-carboxylate, its octylbiphenyl analog, its octyloxycarbonylbiphenyl analog, and 2-fluoro-4-{[(1-trifluoromethyl) undecyloxyl carbonyl) phenyl 4'-(dodecyloxy) biphenyl-4-carboxylate. The heat capacity anomaly around the smectic-A to the chiral-smectic-C transition has been analyzed in detail. It is revealed that the heat anomaly shows a crossover from three-dimensional XY critical to tricritical behavior. All the data are described well with a crossover function which has been obtained by a Rudnick-Nelson type calculation.
引用
收藏
页码:6677 / 6684
页数:8
相关论文
共 43 条
[1]   UNIVERSAL RATIOS AMONG CORRECTION-TO-SCALING AMPLITUDES AND EFFECTIVE CRITICAL EXPONENTS [J].
AHARONY, A ;
AHLERS, G .
PHYSICAL REVIEW LETTERS, 1980, 44 (12) :782-785
[2]   NONASYMPTOTIC CRITICAL-BEHAVIOR FROM FIELD-THEORY AT D=3 - THE DISORDERED-PHASE CASE [J].
BAGNULS, C ;
BERVILLIER, C .
PHYSICAL REVIEW B, 1985, 32 (11) :7209-7231
[3]   LANDAU 2ND-ORDER TO TRICRITICAL CROSSOVER-BEHAVIOR FOR SMECTIC-A SMECTIC-C-ASTERISK TRANSITIONS [J].
CHAN, T ;
BAHR, CH ;
HEPPKE, G ;
GARLAND, CW .
LIQUID CRYSTALS, 1993, 13 (05) :667-675
[4]   NOVEL PHASES EXHIBITING TRISTABLE SWITCHING [J].
CHANDANI, ADL ;
OUCHI, Y ;
TAKEZOE, H ;
FUKUDA, A ;
TERASHIMA, K ;
FURUKAWA, K ;
KISHI, A .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 2-LETTERS & EXPRESS LETTERS, 1989, 28 (07) :L1261-L1264
[5]   SOME REMARKS ON POLYMORPHISM OF SMECTICS [J].
DEGENNES, PG .
MOLECULAR CRYSTALS AND LIQUID CRYSTALS, 1973, 21 (1-2) :49-76
[6]   Crossover from XY critical to tricritical behavior of heat capacity at the smectic-A-chiral-smectic-C liquid-crystal transition [J].
Ema, K ;
Ogawa, M ;
Takagi, A ;
Yao, H .
PHYSICAL REVIEW E, 1996, 54 (01) :R25-R28
[7]   CRITICAL-BEHAVIOR OF HEAT-CAPACITY AT THE SMECTIC-C-ASTERISK(ALPHA)-SMECTIC-A TRANSITION OF THE ANTIFERROELECTRIC LIQUID-CRYSTAL METHYLHEPTYLOXYCARBONYLPHENYL OCTYLOXYBIPHENYL CARBOXYLATE (MHPOBC) [J].
EMA, K ;
WATANABE, J ;
TAKAGI, A ;
YAO, H .
PHYSICAL REVIEW E, 1995, 52 (01) :1216-1219
[8]   Gaussian tricritical behavior of heat capacity at the smectic-A smectic-C liquid crystal transition [J].
Ema, K ;
Takagi, A ;
Yao, H .
PHYSICAL REVIEW E, 1996, 53 (04) :R3036-R3039
[9]   COMPLEX CALORIMETER WITH AC-MODE AND RELAXATION-MODE OPERATION [J].
EMA, K ;
UEMATSU, T ;
SUGATA, A ;
YAO, H .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS SHORT NOTES & REVIEW PAPERS, 1993, 32 (04) :1846-1850
[10]   Gaussian tricritical behavior of heat capacity at the smectic-A-smectic-C liquid crystal transition in a racemic mixture of 4-(1-methylheptyloxycarbonyl)phenyl 4'-octyloxybiphenyl-4-carboxylate [J].
Ema, K ;
Takagi, A ;
Yao, H .
PHYSICAL REVIEW E, 1997, 55 (01) :508-513