Nonlinear response for time-dependent external fields

被引:20
作者
Petravic, J
Evans, DJ
机构
[1] Research School of Chemistry, Australian National University, 0200, Canberra, Australian Capital Territory
关键词
D O I
10.1103/PhysRevLett.78.1199
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We generalize nonlinear response theory for autonomous systems so that it describes the response of classical many-body systems to large time-dependent external fields. Our formalism represents the first practical application of response theory to such problems. Our expressions for the nonlinear time-dependent response are tested against nonequilibrium molecular dynamics computer simulation. The relation of our results to known special cases (time-dependent linear response and time-independent nonlinear response) is discussed.
引用
收藏
页码:1199 / 1202
页数:4
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