Atomic-scale surface control and second-harmonic generation in GdxY1-xCa4O(BO3)3 thin films grown by combinatorial laser molecular-beam epitaxy

被引:4
作者
Kim, TW
Arai, N
Koinuma, H
Matsumoto, Y
Yoshimura, M
Furuya, H
Nakao, H
Mori, Y
Sasaki, T
机构
[1] Tokyo Inst Technol, Frontier Collaborat Res Ctr Lab, Yokohama, Kanagawa 2268503, Japan
[2] Tokyo Inst Technol, Mat & Struct Lab, Midori Ku, Yokohama, Kanagawa 226, Japan
[3] Osaka Univ, Grad Sch Engn, Dept Elect Engn, Suita, Osaka 5650871, Japan
[4] Japan Sci & Tecnol Corp, CREST, Tokyo, Japan
[5] Sci & Technol Agcy Japan, COMET, Tokyo, Japan
关键词
D O I
10.1063/1.1402964
中图分类号
O59 [应用物理学];
学科分类号
摘要
We studied the atomic-scale, growth control and second-harmonic generation (SHG) properties of GdxY1-xCa4O(BO3)(3) thin films. Combinatorial laser molecular-beam epitaxy was employed to optimize the growth conditions of the film. Ultrasmooth GdxY1-xCa4O(BO3)(3) thin films with step-and-terrace structure were obtained by using atomically controlled GdCa4O(BO3)(3) substrates. The dependence of SHG intensity on the fundamental wave polarization angle was studied for the epitaxial film on (010) GdCa4O(BO3)(3) substrate in comparison for the randomly oriented film on (0001) sapphire substrate. It was found that only the epitaxially grown film clearly exhibited a fourfold SHG intensity showing type-II phase-matching direction. (C) 2001 American Institute Of Physics.
引用
收藏
页码:1783 / 1785
页数:3
相关论文
共 15 条
[1]   Linear- and nonlinear-optical properties of a new gadolinium calcium oxoborate crystal, Ca4GdO(BO3)(3) [J].
Aka, G ;
KahnHarari, A ;
Mougel, F ;
Vivien, D ;
Salin, F ;
Coquelin, P ;
Colin, P ;
Pelenc, D ;
Damelet, JP .
JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 1997, 14 (09) :2238-2247
[2]   Crystal growth and characterization of GdxY1-xCa4O(BO3)3 crystal [J].
Furuya, H ;
Yoshimura, M ;
Kobayasbi, T ;
Murase, K ;
Mori, Y ;
Sasaki, T .
JOURNAL OF CRYSTAL GROWTH, 1999, 198 :560-563
[3]   Crystal growth and optical characterization of rare-earth (Re) calcium oxyborate ReCa1O(BO3)(3) (Re=Y or Gd) as new nonlinear optical material [J].
Iwai, M ;
Kobayashi, T ;
Furuya, H ;
Mori, Y ;
Sasaki, T .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 2-LETTERS, 1997, 36 (3A) :L276-L279
[4]   ATOMIC CONTROL OF THE SRTIO3 CRYSTAL-SURFACE [J].
KAWASAKI, M ;
TAKAHASHI, K ;
MAEDA, T ;
TSUCHIYA, R ;
SHINOHARA, M ;
ISHIYAMA, O ;
YONEZAWA, T ;
YOSHIMOTO, M ;
KOINUMA, H .
SCIENCE, 1994, 266 (5190) :1540-1542
[5]  
Kim T.-H., UNPUB
[6]   Growth and ultraviolet application of Li2B4O7 crystals: Generation of the fourth and fifth harmonics of Nd:Y3Al5O12 lasers [J].
Komatsu, R ;
Sugawara, T ;
Sassa, K ;
Sarukura, N ;
Liu, Z ;
Izumida, S ;
Segawa, Y ;
Uda, S ;
Fukuda, T ;
Yamanouchi, K .
APPLIED PHYSICS LETTERS, 1997, 70 (26) :3492-3494
[7]  
KOUTA H, 1993, J CRYST GROWTH, V144, P676
[8]   Growth mode mapping of SrTiO3 epitaxy [J].
Lippmaa, M ;
Nakagawa, N ;
Kawasaki, M ;
Ohashi, S ;
Koinuma, H .
APPLIED PHYSICS LETTERS, 2000, 76 (17) :2439-2441
[9]  
Moloney J. V., 1998, NONLINEAR OPTICAL MA
[10]   NEW NONLINEAR-OPTICAL CRYSTAL - CESIUM LITHIUM BORATE [J].
MORI, Y ;
KURODA, I ;
NAKAJIMA, S ;
SASAKI, T ;
NAKAI, S .
APPLIED PHYSICS LETTERS, 1995, 67 (13) :1818-1820