An investigation into the origins of a series of PM10 anomalies at a remote location in NW England

被引:5
作者
Ferranti, Emma J. S. [1 ]
Whyatt, James Duncan [1 ]
Davison, Brian [2 ]
机构
[1] Univ Lancaster, Dept Geog, Lancaster Environm Ctr, Lancaster LA1 4YQ, England
[2] Univ Lancaster, Lancaster LA1 4YQ, England
来源
JOURNAL OF ENVIRONMENTAL MONITORING | 2008年 / 10卷 / 09期
关键词
D O I
10.1039/b807531j
中图分类号
O65 [分析化学];
学科分类号
070302 [分析化学]; 081704 [应用化学];
摘要
Throughout 2004, PM(10) concentrations were measured at 10 min intervals at Hazelrigg, a remote location in NW England. The annual mean concentration was 6.1 mu g m(-3) and likely origins were determined using directional and particle size characteristics. The fine temporal resolution of the monitoring also allowed several short periods (< 20 h) of persistently high PM(10) concentration to be identified and then 'typed' by event start time, duration, wind direction and particle size characteristics. A series of night time PM(10) anomalies (concentration < 465 mu g m(-3)) of no obvious source were identified, and by elimination assumed to have originated from a ground-based fire of particle-rich fodder. A novel methodology combining Stokes' Law with systematic and rigorous modelling of source strength (using ADMS3.2) was developed to locate a possible burn site. The process was limited by the lack of previous modelling studies related to ground-based fires, and also by the capacity of ADMS3.2 to model sub-hourly time-varying emissions and fluctuations in wind speed and direction in the near field. However, modelling did suggest the source was located < 400 m SSE of Hazelrigg, and investigation of this area revealed a burn site where tyres and plastic bags were piled nearby. Few studies have combined directional analysis and modelling to locate a source based on sampled data. This innovative methodology could be used by regulatory bodies to investigate the origins of unidentified PM(10) observed within the particle record.
引用
收藏
页码:1033 / 1040
页数:8
相关论文
共 23 条
[1]
ABBOTT J, 2006, COMMUNICATION
[2]
Air Quality Expert Group (AQEG), 2005, Particulate matter in the United Kingdom
[3]
[Anonymous], 1999, SOURC APP AIRB PART
[4]
[Anonymous], 1998, QUANT EFF AIR POLL H
[5]
[Anonymous], 2011, Workshop Report of the Intergovernmental Panel on Climate Change Workshop on Impacts of Ocean Acidification on Marine Biology and Ecosystems
[6]
*BODC, 2006, UK NAT TID GAUG NETW
[7]
Validation of ADMS against wind tunnel data of dispersion from chemical warehouse fires [J].
Carruthers, DJ ;
Mckeown, AM ;
Hall, DJ ;
Porter, S .
ATMOSPHERIC ENVIRONMENT, 1999, 33 (12) :1937-1953
[8]
*ENT UK LTD, 2006, INC GROUND AIR QUAL
[9]
*EPA, 1995, AP42 COMP AIR POLL E, V1
[10]
Modelling plume rise and dispersion from pool fires [J].
Fisher, BEA ;
Metcalfe, E ;
Vince, I ;
Yates, A .
ATMOSPHERIC ENVIRONMENT, 2001, 35 (12) :2101-2110