Coherent control of terahertz supercontinuum generation in ultrafast laser-gas interactions

被引:710
作者
Kim, K. Y. [1 ]
Taylor, A. J. [1 ]
Glownia, J. H. [1 ]
Rodriguez, G. [1 ]
机构
[1] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA
关键词
D O I
10.1038/nphoton.2008.153
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Frequency mixing an ultrafast-pulse laser's fundamental and second-harmonic fields in semiconductors(1,2), atomic gases(3,4), and on metal surfaces(5) generates a directional electrical current for which the magnitude and polarity depend upon the relative phase between these two fields(1-5). As this current occurs on the timescale of the duration of the laser pulse, in the case of ultrafast lasers (<100 fs), this process can generate electromagnetic radiation at terahertz frequencies. Although such terahertz generation has been observed in semiconductors(6) and air(7-13), the terahertz generation mechanism is not well understood and the terahertz yield has not been optimized. Here, we demonstrate a coherent control scheme to optimize terahertz generation in gases, yielding a new source of high-energy (>5 mu J), super-broadband terahertz radiation (similar to 75 THz) as well as an enhanced accompanying third harmonic. We also present a unifying explanation for such extremely broad electromagnetic radiation generation.
引用
收藏
页码:605 / 609
页数:5
相关论文
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