The first order phase transition and superconductivity in BaNi2As2 single crystals

被引:158
作者
Ronning, F. [1 ]
Kurita, N. [1 ]
Bauer, E. D. [1 ]
Scott, B. L. [1 ]
Park, T. [1 ,2 ]
Klimczuk, T. [1 ,3 ]
Movshovich, R. [1 ]
Thompson, J. D. [1 ]
机构
[1] Los Alamos Natl Lab, Los Alamos, NM 87545 USA
[2] Sungkyunkwan Univ, Dept Phys, Suwon 440746, South Korea
[3] Gdansk Univ Technol, Fac Appl Phys & Math, PL-80952 Gdansk, Poland
关键词
D O I
10.1088/0953-8984/20/34/342203
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
We report the synthesis and physical properties of single crystals of stoichiometric BaNi2As2 that crystallizes in the ThCr2Si2 structure with lattice parameters a = 4.112(4) angstrom and c = 11.54(2) angstrom. The resistivity and heat capacity show a first order phase transition at T-0 = 130 K with a thermal hysteresis of 7 K. The Hall coefficient is weakly temperature dependent from room temperature to 2 K where it has a value of -4 x 10(-10) Omega cm Oe(-1). The resistivity, ac susceptibility, and heat capacity provide evidence for bulk superconductivity at T-c = 0.7 K. The Sommerfeld coefficient at Tc is 11.6 +/- 0.9 mJ mol(-1) K-2. The upper critical field is anisotropic with initial slopes of dH(c2)(c)/ dT = -0.19 T K-1 and dH(c2)(ab)/ dT = -0.40 T K-1, as determined from the resistivity.
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