Global Mortality Attributable to Aircraft Cruise Emissions

被引:145
作者
Barrett, Steven R. H. [1 ]
Britter, Rex E. [1 ]
Waitz, Ian A. [2 ]
机构
[1] Univ Cambridge, Dept Engn, Cambridge CB2 1PZ, England
[2] MIT, Dept Aeronaut & Astronaut, Cambridge, MA 02139 USA
基金
英国工程与自然科学研究理事会;
关键词
PARTICULATE AIR-POLLUTION; UNITED-STATES; INTERCONTINENTAL TRANSPORT; MODEL DESCRIPTION; IMPACT; VISIBILITY; INVENTORY; AEROSOLS; QUALITY; SYSTEM;
D O I
10.1021/es101325r
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Aircraft emissions impact human health though degradation of air quality. The majority of previous analyses of air quality impacts from aviation have considered only landing and takeoff emissions. We show that aircraft cruise emissions impact human health over a hemispheric scale and provide the first estimate of premature mortalities attributable to aircraft emissions globally. We estimate similar to 8000 premature mortalities per year are attributable to aircraft cruise emissions. This represents similar to 80% of the total impact of aviation (where the total includes the effects of landing and takeoff emissions), and similar to 1% of air quality-related premature mortalities from all sources. However, we note that the impact of landing and takeoff emissions is likely to be under-resolved. Secondary H2SO4-HNO3-NH3 aerosols are found to dominate mortality impacts. Due to the altitude and region of the atmosphere at which aircraft emissions are deposited, the extent of transboundary air pollution is particularly strong. For example, we describe how strong zonal westerly winds aloft, the mean meridional circulation around 30-60 degrees N, interaction of aircraft-attributable aerosol precursors with background ammonia, and high population densities in combination give rise to an estimated similar to 3500 premature mortalities per year in China and India combined, despite their relatively small current share of aircraft emissions. Subsidence of aviation-attributable aerosol and aerosol precursors occurs predominantly around the dry subtropical ridge, which results in reduced wet removal of aviation-attributable aerosol. It is also found that aircraft NOx emissions serve to increase oxidation of nonaviation SO2, thereby further increasing the air quality impacts of aviation. We recommend that cruise emissions be explicitly considered in the development of policies, technologies and operational procedures designed to mitigate the air quality impacts of air transportation.
引用
收藏
页码:7736 / 7742
页数:7
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