Phenomenological damping of nonlinear-optical response tensors

被引:49
作者
Andrews, DL [1 ]
Naguleswaran, S
Stedman, GE
机构
[1] Univ E Anglia, Sch Chem Sci, Norwich NR4 7TJ, Norfolk, England
[2] Univ Canterbury, Dept Phys & Astron, Christchurch 1, New Zealand
来源
PHYSICAL REVIEW A | 1998年 / 57卷 / 06期
关键词
D O I
10.1103/PhysRevA.57.4925
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
The damping factors that occur in nonlinear-optical response tensors are commonly assigned signs that depend upon the temporal ordering of the associated photon interactions. However, time-reversal symmetry is satisfied only if all these signs are identical. For example, only then is there a formal equivalence between the amplitudes for second-harmonic generation and parametric down-conversion and only then is electro-optic rotation forbidden in fluids. This correction reflects deficiencies in certain commonly employed semiclassical approaches to nonlinear optics.
引用
收藏
页码:4925 / 4929
页数:5
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