The Electrochemical Reduction of Carbon Dioxide to Formate/Formic Acid: Engineering and Economic Feasibility

被引：470

作者：

Agarwal, Arun S. ^{[1
]}

Zhai, Yumei ^{[1
]}

Hill, Davion ^{[1
]}

Sridhar, Narasi ^{[1
]}

机构：

[1] Det Norske Veritas USA Inc, Res & Innovat, Dublin, OH 43017 USA

来源：

CHEMSUSCHEM | 2011年 / 4卷 / 09期

关键词：

electrochemistry; hydrogen; carbon dioxide; formic acid; renewable resources; GAS-DIFFUSION ELECTRODES; HIGH-PRESSURE; CONTINUOUS REACTOR; CO2; REDUCTION; ETHYLENE; LEAD;

D O I：

10.1002/cssc.201100220

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

The engineering and economic feasibility of large-scale electrochemical reduction of carbon dioxide to formate salts and formic acid is the focus of this Full Paper. In our study we investigated the long-term performance of tin and other proprietary catalysts in the reduction of carbon dioxide to formate/formic acid at a gas/solid/ liquid interface, using a flow-through reactor. The overall economics and energy consumption of the process are evaluated through a value chain analysis. The sensitivity of the net present value of the process to various process parameters is examined.

引用

页码：1301 / 1310

页数：10

共 31 条

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