Intermittent origin of the large violations of the fluctuation-dissipation relations in an aging polymer glass

被引:46
作者
Buisson, L
Ciliberto, S
Garcimartín, A
机构
[1] Ecole Normale Super Lyon, Phys Lab, CNRS, UMR 5672, F-69364 Lyon 07, France
[2] Univ Navarra, Dept Fis, Fac Ciencias, E-31080 Pamplona, Spain
来源
EUROPHYSICS LETTERS | 2003年 / 63卷 / 04期
关键词
D O I
10.1209/epl/i2003-00551-4
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The fluctuation-dissipation relation (FDR) is measured on the dielectric properties of a polymer glass (polycarbonate) in the range 20 mHz-100 Hz. It is found that after a quench below the glass transition temperature, the fluctuation-dissipation theorem is strongly violated. The amplitude and the persistence time of this violation are decreasing functions of frequency. At frequencies larger than 1 Hz it persists for about 3 h. The origin of this violation is a highly intermittent dynamics characterized by large fluctuations. The relevance of these results for recent models of aging dynamics is discussed.
引用
收藏
页码:603 / 609
页数:7
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