Femtosecond laser photoelectron spectroscopy on atoms and small molecules: Prototype studies in quantum control

被引:184
作者
Wollenhaupt, M [1 ]
Engel, V
Baumert, T
机构
[1] Univ Kassel, Inst Phys, D-34132 Kassel, Germany
[2] Univ Wurzburg, Inst Chem Phys, D-97074 Wurzburg, Germany
关键词
multiphoton ionization; strong field excitation; coherent control; wavepacket dynamics;
D O I
10.1146/annurev.physchem.56.092503.141315
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We review prototype studies in the area of quantum control with femtosecond lasers. We restrict this discussion to atoms and diatomics under gas-phase collision-free conditions to allow for a comparison between theory and experiment. Both the perturbative regime and the nonperturbative regime of the light-matter interaction are addressed. To that end, atomic/molecular beam techniques are combined together with femtosecond laser techniques and energy-resolved photoelectron spectroscopy and ion detection. Highly detailed information on the laser-induced quantum dynamics is extracted with the help of kinetic energy-resolved photoelectron spectroscopy.
引用
收藏
页码:25 / 56
页数:32
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