Ultrafast response of third-order optical nonlinearity in glasses containing Bi2O3

被引：100

作者：

Sugimoto, N ^{[1
]}

Kanbara, H ^{[1
]}

Fujiwara, S ^{[1
]}

Tanaka, K ^{[1
]}

Hirao, K ^{[1
]}

机构：

[1] KYOTO UNIV, FAC ENGN, KYOTO 606, JAPAN

来源：

OPTICS LETTERS | 1996年 / 21卷 / 20期

关键词：

D O I：

10.1364/OL.21.001637

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

We prepared nonresonant-type homogeneous glasses containing Bi2O3 by the melting method. The third-order optical nonlinear susceptibility chi((3)) was found by third-order harmonic generation measurement to be 9.3 x 10(-12) esu. We attribute the nonlinearity of these glasses to the large molar refraction of glasses containing Bi2O3 These glasses also exhibited an ultrafast response time below 200 fs by a degenerate four-wave mixing method using a femtosecond laser, indicating that the nonlinearity of these glasses originated mainly from pure electronic polarization. (C) 1996 Optical Society of America

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页码：1637 / 1639

页数：3

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