Plasmonic sensing characteristics of single nanometric holes

被引:219
作者
Rindzevicius, T
Alaverdyan, Y
Dahlin, A
Hook, F
Sutherland, DS
Kall, M [1 ]
机构
[1] Chalmers Univ Technol, Dept Appl Phys, S-41296 Gothenburg, Sweden
[2] Lund Univ, Div Solid State Phys, S-22100 Lund, Sweden
关键词
D O I
10.1021/nl0516355
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The optical response of isolated holes in 20 nm thin gold is probed as a function of alkanethiol CH3(CH2)(x)SH (x is an element of 1-15) and protein adsorption using dark-field spectroscopy. We establish that the plasmon excitations of single and short-range ordered 60 nm holes exhibit similar E-field decay lengths delta approximate to 10-20 nm and that a single hole can be used to resolve the successive adsorption of a protein (biotin-BSA) and its interaction partner (neutravidin). The data confirm the localized character of the hole plasmon and demonstrate that its applicability for bio/chemosensing is similar to that of particle plasmons.
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收藏
页码:2335 / 2339
页数:5
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