Microscopic theory of spin-polarization coupling in multiferroic transition metal oxides

被引:274
作者
Jia, Chenglong [1 ]
Onoda, Shigeki [2 ]
Nagaosa, Naoto [3 ,4 ]
Han, Jung Hoon [5 ,6 ]
机构
[1] Korea Inst Adv Study, Sch Phys, Seoul 130012, South Korea
[2] Inst Phys & Chem Res, RIKEN, Wako, Saitama 3510918, Japan
[3] Univ Tokyo, Dept Appl Phys, CREST, Tokyo 1138656, Japan
[4] Natl Inst Adv Ind Sci & Technol, Correlated Elect Res Ctr, Tsukuba, Ibaraki 3058562, Japan
[5] Sungkyunkwan Univ, Dept Phys, BK21 Phys Res Div, Suwon 440746, South Korea
[6] Seoul Natl Univ, CSCMR, Seoul 151747, South Korea
关键词
D O I
10.1103/PhysRevB.76.144424
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
A systematic microscopic theory of magnetically induced ferroelectricity and lattice modulation is presented for various electron configurations of Mott-insulating transition metal oxides. The origin of polarization is classified as the spin-orbit interaction effective (i) within the magnetic t(2g) orbitals, (ii) between the t(2g) and e(g) orbitals, and (iii) within the ligand ion's p orbitals. Predictions for x-ray and neutron scattering experiments are proposed to clarify the microscopic mechanism of the spin-polarization coupling in different materials. Semiquantitative agreements with the multiferroic TbMnO3 are obtained.
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页数:7
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