SOLEIL a new powerful tool for materials science

被引:20
作者
Baudelet, F
Belkhou, R
Briois, V
Coati, A
Dumas, P
Etgens, VH
Flank, AM
Fontaine, P
Garreau, Y
Lyon, O
Quinkal, I
Rochet, F
Roy, P
Sauvage, M
Sirotti, F
Somogyi, A
Thiaudière, D
机构
[1] Synchrotron SOLEIL, F-91192 Gif Sur Yvette, France
[2] Ctr Univ, LURE, F-91898 Orsay, France
[3] Univ Paris 06, Inst NanoSci Paris, F-75015 Paris, France
[4] Univ Paris 07, Inst NanoSci Paris, F-75015 Paris, France
[5] Lab Chim Phys Mat & Rayonnement, F-75231 Paris, France
来源
OIL & GAS SCIENCE AND TECHNOLOGY-REVUE D IFP ENERGIES NOUVELLES | 2005年 / 60卷 / 05期
关键词
D O I
10.2516/ogst:2005060
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
The first photons delivered by the third generation synchrotron source SOLEIL will be soon available for the scientific community. In this context, this paper presents an overview of the potentialities offered by this new machine for the study of materials. The outstanding brilliance of the SOLEIL source will enable to reduce by several orders of magnitude the data collection time for most of the synchrotron techniques (X-ray absorption spectroscopy - EXAFS, wide and small angle X-ray scattering - WAXS and SAXS, X-ray diffraction XRD, photoelectron spectroscopy and microscopy-XPS and PEEM, etc.) thus allowing an operando approach of catalysis processes. The spatial resolution, from a few micrometers to sub micrometer scale, accessible by microdiffraction and microspectroscopy in the wavelength range from the jar IR to the hard X-rays, will provide spatial distributions of different elements (atomic and chemical state selectivity) in a material, from the working heterogeneous catalyst to the reservoir rocks. The reactivity of sulfaces and nanoparticles exposed to controlled gasfluxes will be studied by several in situ techniques. Finally the combination of different synchrotron techniques (diffraction, absorption and fluorescence X) and the access to complementary information obtained through the simultaneous combination of these techniques with those routinely applied in Materials Science, such as UV-Vis or Raman spectroscopy, will offer enlarged capabilities for the operando characterization of materials.
引用
收藏
页码:849 / 874
页数:26
相关论文
共 103 条
[1]   Tuning surface reactivity via electron quantum confinement [J].
Aballe, L ;
Barinov, A ;
Locatelli, A ;
Heun, S ;
Kiskinova, M .
PHYSICAL REVIEW LETTERS, 2004, 93 (19) :196103-1
[2]   Hydrogenation of carbon monoxide on Ni(111) investigated with surface X-ray diffraction at atmospheric pressure [J].
Ackermann, M ;
Robach, O ;
Walker, C ;
Quiros, C ;
Isern, H ;
Ferrer, S .
SURFACE SCIENCE, 2004, 557 (1-3) :21-30
[3]  
ADE H, 2000, CHEM APPL SYNCHROTRO
[4]   Nucleation and initial growth of platinum islands by plasma sputter deposition [J].
Andreazza, P ;
Andreazza-Vignolle, C ;
Rozenbaum, JP ;
Thomann, AL ;
Brault, P .
SURFACE & COATINGS TECHNOLOGY, 2002, 151 :122-127
[5]  
Areán CO, 1999, PHYS CHEM CHEM PHYS, V1, P4139
[6]   Grazing incidence small-angle X-ray scattering of BN-Fe and BN-Ag nanocomposite films obtained by cosputtering and multilayer deposition techniques [J].
Babonneau, D ;
Camelio, S ;
Girardeau, T ;
Jaouen, M ;
Lyon, O .
JOURNAL OF APPLIED CRYSTALLOGRAPHY, 2003, 36 (01) :430-434
[7]   Morphology of encapsulated iron nanoparticles obtained by co-sputtering and implantation: a GISAXS study [J].
Babonneau, D ;
Naudon, A ;
Cabioc'h, T ;
Lyon, O .
JOURNAL OF APPLIED CRYSTALLOGRAPHY, 2000, 33 (01) :437-441
[8]   Direct observation of surface chemistry using ultrafast soft-x-ray pulses [J].
Bauer, M ;
Lei, C ;
Read, K ;
Tobey, R ;
Gland, J ;
Murnane, MM ;
Kapteyn, HC .
PHYSICAL REVIEW LETTERS, 2001, 87 (02) :1-025501
[9]  
Bazin D, 2004, STUD SURF SCI CATAL, V147, P343
[10]   X-ray absorption spectroscopy and anomalous wide angle X-ray scattering: Two basic tools in the analysis of heterogeneous catalysts [J].
Bazin, D ;
Lynch, J ;
Rarnos-Fernandez, M .
OIL & GAS SCIENCE AND TECHNOLOGY-REVUE D IFP ENERGIES NOUVELLES, 2003, 58 (06) :667-683