Role of nuclear rotation in dissociation of H2+ in a short laser pulse

被引:51
作者
Anis, Fatima [1 ]
Esry, B. D. [1 ]
机构
[1] Kansas State Univ, JR Macdonald Lab, Manhattan, KS 66506 USA
来源
PHYSICAL REVIEW A | 2008年 / 77卷 / 03期
关键词
D O I
10.1103/PhysRevA.77.033416
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We revisit the problem of H-2(+) in an intense, short laser pulse to investigate the role of nuclear rotation and thus gauge the validity of the more common aligned molecule approximation. For the laser parameters considered, our results show rough qualitative agreement, but not quantitative agreement. In one case, however, the aligned molecule approximation deviates even qualitatively from the more complete calculation by overestimating the importance of vibrational trapping.
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页数:11
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共 28 条
[1]   Dynamical quenching of laser-induced dissociations of diatomic molecules in intense infrared fields: Effects of molecular rotations and misalignments [J].
Abou-Rachid, H ;
Nguyen-Dang, TT ;
Atabek, O .
JOURNAL OF CHEMICAL PHYSICS, 2001, 114 (05) :2197-2207
[2]   Simultaneous real-time tracking of wave packets evolving on two different potential curves in H+2 + and D2+ -: art. no. 030702 [J].
Alnaser, AS ;
Ulrich, B ;
Tong, XM ;
Litvinyuk, IV ;
Maharjan, CM ;
Ranitovic, P ;
Osipov, T ;
Ali, R ;
Ghimire, S ;
Chang, Z ;
Lin, CD ;
Cocke, CL .
PHYSICAL REVIEW A, 2005, 72 (03)
[3]   Laser-assisted charge transfer in He2++H collisions -: art. no. 043414 [J].
Anis, F ;
Roudnev, V ;
Cabrera-Trujillo, R ;
Esry, BD .
PHYSICAL REVIEW A, 2006, 73 (04)
[4]   MOLECULAR STABILIZATION AND ANGULAR-DISTRIBUTION IN PHOTODISSOCIATION OF H-2+ IN INTENSE LASER FIELDS [J].
AUBANEL, EE ;
GAUTHIER, JM ;
BANDRAUK, AD .
PHYSICAL REVIEW A, 1993, 48 (03) :2145-2152
[5]   EFFECT OF ROTATIONS ON STABILIZATION IN HIGH-INTENSITY PHOTODISSOCIATION OF H-2+ [J].
AUBANEL, EE ;
CONJUSTEAU, A ;
BANDRAUK, AD .
PHYSICAL REVIEW A, 1993, 48 (06) :R4011-R4014
[6]   Classical aspects of ultracold atom wave packet motion through microstructured waveguide bends [J].
Bromley, MWJ ;
Esry, BD .
PHYSICAL REVIEW A, 2004, 69 (05) :053620-1
[7]   FRAGMENT ANGULAR-DISTRIBUTION IN ONE-COLOR AND 2-COLOR PHOTODISSOCIATION BY STRONG LASER FIELDS [J].
CHARRON, E ;
GIUSTISUZOR, A ;
MIES, FH .
PHYSICAL REVIEW A, 1994, 49 (02) :R641-R644
[8]   Dynamical quenching of field-induced dissociation of H2+ in intense infrared lasers [J].
Châteauneuf, F ;
Nguyen-Dang, TT ;
Ouellet, N ;
Atabek, O .
JOURNAL OF CHEMICAL PHYSICS, 1998, 108 (10) :3974-3986
[9]   Time-dependent studies of single and multiple photoionization of H2+ -: art. no. 063413 [J].
Colgan, J ;
Pindzola, MS ;
Robicheaux, F .
PHYSICAL REVIEW A, 2003, 68 (06) :9
[10]   Spatiotemporal imaging of ultrafast molecular motion:: Collapse and revival of the D2+ nuclear wave packet [J].
Ergler, Th. ;
Rudenko, A. ;
Feuerstein, B. ;
Zrost, K. ;
Schroeter, C. D. ;
Moshammer, R. ;
Ullrich, J. .
PHYSICAL REVIEW LETTERS, 2006, 97 (19)