Comparison of Pu and 137Cs as tracers of soil and sediment transport in a terrestrial environment

Following atmospheric nuclear weapons testing in the 1950s and 1960s significant quantities of (CS)-C-137 and Pu239+240 were deposited worldwide. In recent decades, Cs-137 has been commonly used as a tracer of soil erosion and sedimentation, particularly in the Northern Hemisphere where atomic deposition was three times as great as in the Southern Hemisphere. The relatively short 30-year half-life of this isotope means that its sensitivity as a tracer is rapidly decreasing. In contrast, with half-lives of 24,110 and 6561 years, the sensitivity of the two plutonium isotopes remains essentially the same as when it was deposited. Here we use the technique of Accelerator Mass Spectrometry to demonstrate the potential of anthropogenic Pu as an alternative to 137Cs as a tracer of soil transport in Australia. We measure an average Cs-137/Pu239+240 activity ratio of 27.3 +/- 1.5 and an average Pu-240/Pu-239 atom ratio of 0.149 +/- 0.003, both slightly lower than the global average. (C) 2007 Elsevier Ltd. All rights reserved.