CO2 reforming of methane by the combination of dielectric-barrier discharges and catalysis

被引：188

作者：

Kraus, M ^{[1
]}

Eliasson, B

Kogelschatz, U

Wokaun, A

机构：

[1] Paul Scherrer Inst, CH-5232 Villigen, Switzerland

[2] ABB Corp Res Ltd, CH-5405 Baden, Switzerland

来源：

PHYSICAL CHEMISTRY CHEMICAL PHYSICS | 2001年 / 3卷 / 03期

关键词：

D O I：

10.1039/b007015g

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The combination of solid state catalysts with a dielectric-barrier discharge was studied for the CO2 reforming of methane, including the methane and carbon dioxide decomposition reactions. Nickel and rhodium coatings were investigated for their influence on the plasma chemical reactions. It is shown that the use of a catalytic coating in the discharge can have a promoting effect on the plasma chemistry. Secondly, the use of the ceramic foams improved the temperature control in the discharge and lowered the undesired temperature increase in the discharge.

引用

页码：294 / 300

页数：7

共 22 条

[1]

Bodrov I. M., 1967, KINET KATAL, V8, P379

[2]

Brook SL, 1998, J CATAL, V180, P225

[3] THE CHEMISTRY OF METHANE REFORMING WITH CARBON-DIOXIDE AND ITS CURRENT AND POTENTIAL APPLICATIONS [J].