Internal laser-induced dipole force at work in C60 molecule -: art. no. 203004

被引:128
作者
Bhardwaj, VR [1 ]
Corkum, PB [1 ]
Rayner, DM [1 ]
机构
[1] Natl Res Council Canada, Steacie Inst Mol Sci, Ottawa, ON K1A 0R6, Canada
关键词
D O I
10.1103/PhysRevLett.91.203004
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We show how the many electron response of a complex molecule to an intense laser field can be incorporated with the single active electron picture. This enables us to introduce an "over-the-barrier" model for C-60(z+) ionization, valid for long wavelength light. Using infrared radiation, we confirm the model and also produce stable, highly charged C-60 reaching C-60(12+), the highest charge state ever observed. At high intensities and high charge states the internal laser-induced dipole force and rapid charging lead to stress on the molecule. The interplay between the forces provides control and suggest strategies for reaching even higher charge states.
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页数:4
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