Dynamic processes of mercury over the Mediterranean region: results from the Mediterranean Atmospheric Mercury Cycle System (MAMCS) project

被引:48
作者
Pirrone, N [1 ]
Ferrara, R
Hedgecock, IM
Kallos, G
Mamane, Y
Munthe, J
Pacyna, JM
Pytharoulis, I
Sprovieri, F
Voudouri, A
Wangberg, I
机构
[1] CNR, Inst Atmospher Pollut, I-87036 Arcavacata Di Rende, Italy
[2] CNR, Inst Biophys, I-56100 Pisa, Italy
[3] Univ Athens, Sch Phys, Athens, Greece
[4] Technion Israel Inst Technol, Haifa, Israel
[5] Swedish Environm Res Inst, S-40258 Gothenburg, Sweden
[6] Norwegian Inst Air Res, Kjeller, Norway
关键词
mercury; cycling; measurements; modelling; Mediterranean Sea; atmosphere;
D O I
10.1016/S1352-2310(03)00251-6
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The Mediterranean Atmospheric Mercury Cycle System (MAMCS) project was performed between 1998 and 2000 and involved the collaboration of universities and research institutes from Europe, Israel and Turkey. The main goal of MAMCS was to investigate dynamic processes affecting the cycle of mercury in the Mediterranean atmosphere by combining Lid hoc field measurements and modelling tasks. To study the fate of Hg in the Mediterranean Basin an Updated emission inventory was compiled for Europe and the Countries bordering the Mediterranean Sea. Models were developed to describe the individual atmospheric processes which influence the chemical and physical characteristics of atmospheric Ha. and these were coupled to meteorological models to examine the dispersion and deposition of Hg species in the Mediterranean Basin. One intercomparison and four two-week measurement campaigns were carried out over a three-year period. The work presented here describes the results in general terms but focuses Oil the areas where definite conclusions were unforthcoming and thus highlights those aspects where, in spite of advances made in the understanding of Ha cycling, further work is necessary in order to be able to predict confidently Hg and Hg compound concentration fields and deposition patterns. (C) 2003 Elsevier Science Ltd. All rights reserved.
引用
收藏
页码:S21 / S39
页数:19
相关论文
共 52 条
[1]  
Alpert P., 1990, Tellus, Series A (Dynamic Meteorology and Oceanography), V42A, P65, DOI 10.1034/j.1600-0870.1990.00007.x
[2]   DETERMINATION OF VOLATILE MERCURY SPECIES AT THE PICOGRAM LEVEL BY LOW-TEMPERATURE GAS-CHROMATOGRAPHY WITH COLD-VAPOR ATOMIC FLUORESCENCE DETECTION [J].
BLOOM, N ;
FITZGERALD, WF .
ANALYTICA CHIMICA ACTA, 1988, 208 (1-2) :151-161
[3]   THE BEHAVIOR OF MERCURY IN THE PHYSICAL-ENVIRONMENT [J].
BROSSET, C .
WATER AIR AND SOIL POLLUTION, 1987, 34 (02) :145-166
[5]  
ELFANDY MG, 1946, J ROYAL METEOROLOGIC, V72, P291
[6]   Temporal trends in gaseous mercury evasion from the Mediterranean seawaters [J].
Ferrara, R ;
Mazzolai, B ;
Lanzillotta, E ;
Nucaro, E ;
Pirrone, N .
SCIENCE OF THE TOTAL ENVIRONMENT, 2000, 259 (1-3) :183-190
[7]   Elemental gas phase atmospheric mercury as it interacts with the ambient aerosol and its subsequent speciation and deposition [J].
Forlano, L ;
Hedgecock, IM ;
Pirrone, N .
SCIENCE OF THE TOTAL ENVIRONMENT, 2000, 259 (1-3) :211-222
[8]   Mercury and photochemistry in the marine boundary layer-modelling studies suggest the in situ production of reactive gas phase mercury [J].
Hedgecock, IM ;
Pirrone, N .
ATMOSPHERIC ENVIRONMENT, 2001, 35 (17) :3055-3062
[9]  
JANJIC ZI, 1994, MON WEATHER REV, V122, P927, DOI 10.1175/1520-0493(1994)122<0927:TSMECM>2.0.CO
[10]  
2