Supercooled liquids and glasses

被引:1949
作者
Ediger, MD
Angell, CA
Nagel, SR
机构
[1] ARIZONA STATE UNIV, DEPT CHEM, TEMPE, AZ 85287 USA
[2] UNIV CHICAGO, JAMES FRANCK INST, CHICAGO, IL 60637 USA
[3] UNIV CHICAGO, DEPT PHYS, CHICAGO, IL 60637 USA
关键词
D O I
10.1021/jp953538d
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Selected aspects of recent progress in the study of supercooled liquids and glasses are presented in this review. As an introduction for nonspecialists, several basic features of the dynamics and thermodynamics of supercooled liquids and glasses are described. Among these are nonexponential relaxation functions, non-Arrhenius temperature dependences, and the Kauzmann temperature. Various theoretical models which attempt to explain these basic features are presented next. These models are conveniently categorized according to the temperature regimes deemed important by their authors. The major portion of this review is given to a summary of current experimental and computational research. The utility of mode coupling theory is addressed. Evidence is discussed for new relaxation mechanisms and new time and length scales in supercooled liquids. Relaxations in the glassy state and significance of the ''boson peak'' are also addressed.
引用
收藏
页码:13200 / 13212
页数:13
相关论文
共 155 条
  • [1] DIELECTRIC RELAXATIONS IN VARIOUS CRYSTAL MODIFICATIONS OF CYCLOHEXANOL AND 2,3-DIMETHYLBUTANE
    ADACHI, K
    SEKI, S
    WADA, Y
    SUGA, H
    YAMAGUCHI, S
    YANO, O
    KUBOTA, S
    [J]. MOLECULAR CRYSTALS AND LIQUID CRYSTALS, 1972, 18 (3-4) : 345 - +
  • [2] ON TEMPERATURE DEPENDENCE OF COOPERATIVE RELAXATION PROPERTIES IN GLASS-FORMING LIQUIDS
    ADAM, G
    GIBBS, JH
    [J]. JOURNAL OF CHEMICAL PHYSICS, 1965, 43 (01) : 139 - &
  • [3] ALPHA-RELAXATION IN THE GLASS-TRANSITION RANGE OF AMORPHOUS POLYMERS .1. TEMPERATURE BEHAVIOR ACROSS THE GLASS-TRANSITION
    ALEGRIA, A
    GUERRICAECHEVARRIA, E
    GOITIANDIA, L
    TELLERIA, I
    COLMENERO, J
    [J]. MACROMOLECULES, 1995, 28 (05) : 1516 - 1527
  • [4] NON-DEBYE DIELECTRIC-RELAXATION AROUND THE LIQUID-GLASS TRANSITION OF A GLASS-FORMING POLYMER
    ALEGRIA, A
    GUERRICAECHEVARRIA, E
    TELLERIA, I
    COLMENERO, J
    [J]. PHYSICAL REVIEW B, 1993, 47 (22): : 14857 - 14865
  • [5] CONFIGURATIONAL EXCITATIONS IN CONDENSED MATTER, AND BOND LATTICE MODEL FOR LIQUID-GLASS TRANSITION
    ANGELL, CA
    RAO, KJ
    [J]. JOURNAL OF CHEMICAL PHYSICS, 1972, 57 (01) : 470 - &
  • [6] ANGELL CA, 1992, AIP CONF PROC, V256, P3, DOI 10.1063/1.42338
  • [7] PERSPECTIVE ON THE GLASS-TRANSITION
    ANGELL, CA
    [J]. JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS, 1988, 49 (08) : 863 - 871
  • [8] FAST ION MOTION IN GLASSY AND AMORPHOUS MATERIALS
    ANGELL, CA
    [J]. SOLID STATE IONICS, 1983, 9-10 (DEC) : 3 - 16
  • [9] STRONG AND FRAGILE PLASTIC CRYSTALS
    ANGELL, CA
    DWORKIN, A
    FIGUIERE, P
    FUCHS, A
    SZWARC, H
    [J]. JOURNAL DE CHIMIE PHYSIQUE ET DE PHYSICO-CHIMIE BIOLOGIQUE, 1985, 82 (7-8) : 773 - 777
  • [10] DYNAMIC PROCESSES IN IONIC GLASSES
    ANGELL, CA
    [J]. CHEMICAL REVIEWS, 1990, 90 (03) : 523 - 542