Electronic excited states of NO/Cu(111) studied by high-resolution two-photon photoelectron spectroscopy

被引:6
作者
Munakata, T [1 ]
Sakashita, T [1 ]
Tsukakoshi, M [1 ]
Nakamura, J [1 ]
机构
[1] SCI UNIV TOKYO, SHINJUKU KU, TOKYO 162, JAPAN
关键词
copper; nitrogen oxides; surface electronic phenomena; visible and ultraviolet photoelectron spectroscopy;
D O I
10.1016/0039-6028(96)00235-X
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A high-resolution two-photon photoelectron (2PPE) spectrometer was constructed and applied to NO adsorbed Cu(111). The apparatus was based on a high-repetitive tunable laser of picosecond pulse duration combined with a single-electron counting time-of-flight (TOF) system. Performance of the apparatus was examined with 2PPE spectra of Ag(111) and Cu(111) surfaces, Energy resolution better than 0.03 eV was achieved. A preliminary result for NO adsorbed Cu(111) surface showed that electronic states of adsorbed NO contain some fine structures, suggesting that the high-resolution 2PPE spectroscopy provides much information on electronic structure of adsorbed molecules.
引用
收藏
页码:629 / 633
页数:5
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