Photoelectron diffraction mapping:: Molecules illuminated from within -: art. no. 013002

被引：163

作者：

Landers, A ^{[1
]}

Weber, T

Ali, I

Cassimi, A

Hattass, M

Jagutzki, O

Nauert, A

Osipov, T

Staudte, A

Prior, MH

Schmidt-Böcking, H

Cocke, CL

Dörner, R

机构：

[1] Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA

[2] Univ Frankfurt, Inst Kernphys, D-60486 Frankfurt, Germany

[3] Kansas State Univ, Dept Phys, Manhattan, KS 66506 USA

[4] Univ Caen, ISMRA, CNRS, CEA,CIRIL, F-14070 Caen 5, France

[5] Univ Calif Berkeley, Lawrence Berkeley Lab, Div Chem Sci, Berkeley, CA 94720 USA

[6] Univ Freiburg, Fak Phys, D-79104 Freiburg, Germany

来源：

PHYSICAL REVIEW LETTERS | 2001年 / 87卷 / 01期

关键词：

D O I：

10.1103/PhysRevLett.87.013002

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

We demonstrate the use of a multiparticle coincidence technique to image the diffraction of an electron wave whose source is placed at a specific site in a free molecule. Core-level photoelectrons are used to illuminate the molecule from within. By measuring the vector momenta of two molecular fragments and the photoelectron, a richly structured electron diffraction pattern is obtained in a body-fixed frame of the randomly oriented molecule in the gas phase. We illustrate this technique for CO, creating a photoelectron from the C(1s) shell and scanning its energy from zero to 30 eV.

引用

页数：4

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