A powerful approach to fabricate nitrogen-doped graphene sheets with high specific surface area

被引：92

作者：

Yang, Shin-Yi

Chang, Kuo-Hsin

Huang, Yuan-Li

Lee, Ying-Feng

Tien, Hsi-Wen

Li, Shin-Ming

Lee, Ying-Hui

Liu, Chia-Hong

Ma, Chen-Chi M. ^{[1
]}

Hu, Chi-Chang

机构：

[1] Natl Tsing Hua Univ, Dept Chem Engn, Hsinchu 30013, Taiwan

来源：

ELECTROCHEMISTRY COMMUNICATIONS | 2012年 / 14卷 / 01期

关键词：

Nitrogen-doped graphene sheet; Electrocatalyst; Oxygen reduction reaction; HIGH ELECTROCATALYTIC ACTIVITY; OXYGEN-REDUCTION ACTIVITY; ELECTROCHEMICAL PERFORMANCE; CARBON ELECTRODES; FUNCTIONAL-GROUPS; GRAPHITE OXIDE; ARRAYS; IRON;

D O I：

10.1016/j.elecom.2011.10.028

中图分类号：

O646 [电化学、电解、磁化学];

学科分类号：

081704 ;

摘要：

This study develops a powerful strategy for fabricating the nitrogen-doped graphene sheets with good crystallinity, high specific surface area, and high percentages of pyridinic/graphitic-nitrogen structures. Due to the specified N-doping structures and high specific surface area of 719 m(2) g(-1), our N-doped graphene sheets show an excellent electrocatalytic activity for the oxygen reduction reaction (ORR). (C) 2011 Elsevier B.V. All rights reserved.

引用

收藏

页码：39 / 42

页数：4

相关论文

共 36 条

[1] Electroreduction of oxygen on nitrogen-doped carbon nanotube modified glassy carbon electrodes in acid and alkaline solutions [J].

Alexeyeva, N. ;

Shulga, E. ;

Kisand, V. ;

Kink, I. ;

Tammeveski, K. .

JOURNAL OF ELECTROANALYTICAL CHEMISTRY, 2010, 648 (02) :169-175

[2] Toward N-Doped Graphene via Solvothermal Synthesis [J].

Deng, Dehui ;

Pan, Xiulian ;

Yu, Liang ;

Cui, Yi ;

Jiang, Yeping ;

Qi, Jing ;

Li, Wei-Xue ;

Fu, Qiang ;

Ma, Xucun ;

Xue, Qikun ;

Sun, Gongquan ;

Bao, Xinhe .

CHEMISTRY OF MATERIALS, 2011, 23 (05) :1188-1193

[3] Chemically Derived Graphene Oxide: Towards Large-Area Thin-Film Electronics and Optoelectronics [J].

Eda, Goki ;

Chhowalla, Manish .

ADVANCED MATERIALS, 2010, 22 (22) :2392-2415

[4] Electrocatalytic reduction of oxygen at Au nanoparticles-manganese oxide nanoparticle binary catalysts [J].

El-Deab, Mohamed S. ;

Ohsaka, Takeo .

JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2006, 153 (07) :A1365-A1371

[5] High oxygen-reduction activity and durability of nitrogen-doped graphene [J].

Geng, Dongsheng ;

Chen, Ying ;

Chen, Yougui ;

Li, Yongliang ;

Li, Ruying ;

Sun, Xueliang ;

Ye, Siyu ;

Knights, Shanna .

ENERGY & ENVIRONMENTAL SCIENCE, 2011, 4 (03) :760-764

[6] Nitrogen-Doped Carbon Nanotube Arrays with High Electrocatalytic Activity for Oxygen Reduction [J].

Gong, Kuanping ;

Du, Feng ;

Xia, Zhenhai ;

Durstock, Michael ;

Dai, Liming .

SCIENCE, 2009, 323 (5915) :760-764

[7] Electrochemical performance of nitrogen-enriched carbons in aqueous and non-aqueous supercapacitors [J].

Hulicova, D ;

Kodama, M ;

Hatori, H .

CHEMISTRY OF MATERIALS, 2006, 18 (09) :2318-2326

[8] Nitrogen-Enriched Nonporous Carbon Electrodes with Extraordinary Supercapacitance [J].

Hulicova-Jurcakova, Denisa ;

Kodama, Masaya ;

Shiraishi, Soshi ;

Hatori, Hiroaki ;

Zhu, Zong Hua ;

Lu, Gao Qing .

ADVANCED FUNCTIONAL MATERIALS, 2009, 19 (11) :1800-1809

[9] Combined Effect of Nitrogen- and Oxygen-Containing Functional Groups of Microporous Activated Carbon on its Electrochemical Performance in Supercapacitors [J].

Hulicova-Jurcakova, Denisa ;

Seredych, Mykola ;

Lu, Gao Qing ;

Bandosz, Teresa J. .

ADVANCED FUNCTIONAL MATERIALS, 2009, 19 (03) :438-447

[10] Oxygen-reduction activity of silk-derived carbons [J].

Iwazaki, Tomoya ;

Yang, Hongsheng ;

Obinata, Ryoujin ;

Sugimoto, Wataru ;

Takasu, Yoshio .

JOURNAL OF POWER SOURCES, 2010, 195 (18) :5840-5847

← 1 2 3 4 →