Solubility of single gases carbon dioxide and hydrogen sulfide in aqueous solutions of N-methyldiethanolamine at temperatures from 313 to 393 K and pressures up to 7.6 MPa:: New experimental data and model extension

被引:129
作者
Kamps, APS
Balaban, A
Jödecke, M
Kuranov, G
Smirnova, NA
Maurer, G [1 ]
机构
[1] Univ Kaiserslautern, Lehrstuhl Tech Thermodynam, D-67653 Kaiserslautern, Germany
[2] St Petersburg State Univ, Dept Chem, St Petersburg, Russia
关键词
D O I
10.1021/ie000441r
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
New experimental results for the solubility of the single gases carbon dioxide and hydrogen sulfide in 8 m (i.e., 48.8 wt %) aqueous solutions of 2,2'-methyliminodiethanol (N-methyldiethanolamine; MDEA) at temperatures between 313 and 393 K and total pressures up to 7.6 MPa are reported. A thermodynamic model for describing such phase equilibria is revised and extended using the new data.
引用
收藏
页码:696 / 706
页数:11
相关论文
共 29 条
[1]  
[Anonymous], 1991, ACTIVITY COEFFICIENT, DOI DOI 10.1201/9781351069472
[2]   MODEL OF VAPOR-LIQUID-EQUILIBRIA FOR AQUEOUS ACID GAS-ALKANOLAMINE SYSTEMS .2. REPRESENTATION OF H2S AND CO2 SOLUBILITY IN AQUEOUS MDEA AND CO2 SOLUBILITY IN AQUEOUS MIXTURES OF MDEA WITH MEA OR DEA [J].
AUSTGEN, DM ;
ROCHELLE, GT ;
CHEN, CC .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1991, 30 (03) :543-555
[3]  
Bhairi A. M., 1984, THESIS U OKLAHOMA ST
[4]   THERMODYNAMICS OF ELECTROLYTES .12. DIELECTRIC PROPERTIES OF WATER AND DEBYE-HUCKEL PARAMETERS TO 350-DEGREES-C AND 1-KBAR [J].
BRADLEY, DJ ;
PITZER, KS .
JOURNAL OF PHYSICAL CHEMISTRY, 1979, 83 (12) :1599-1603
[5]   CORRESPONDING STATES CORRELATIONS FOR LIQUID COMPRESSIBILITY AND PARTIAL MOLAL VOLUMES OF GASES AT INFINITE DILUTION IN LIQUIDS [J].
BRELVI, SW ;
OCONNELL, JP .
AICHE JOURNAL, 1972, 18 (06) :1239-&
[6]   SOLUBILITY OF CO2 IN AQUEOUS METHYLDIETHANOLAMINE AND N,N-BIS(HYDROXYETHYL)PIPERAZINE SOLUTIONS [J].
CHAKMA, A ;
MEISEN, A .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1987, 26 (12) :2461-2466
[7]   SOLUBILITY OF CARBON-DIOXIDE IN AQUEOUS MIXTURES OF ALKANOLAMINES [J].
DAWODU, OF ;
MEISEN, A .
JOURNAL OF CHEMICAL AND ENGINEERING DATA, 1994, 39 (03) :548-552
[8]  
Dymond J.H., 1980, VIRIAL COEFFICIENTS
[9]   VAPOR-LIQUID-EQUILIBRIA IN MULTICOMPONENT AQUEOUS-SOLUTIONS OF VOLATILE WEAK ELECTROLYTES [J].
EDWARDS, TJ ;
MAURER, G ;
NEWMAN, J ;
PRAUSNITZ, JM .
AICHE JOURNAL, 1978, 24 (06) :966-976
[10]   GENERALIZED METHOD FOR PREDICTING 2ND VIRIAL-COEFFICIENTS [J].
HAYDEN, JG ;
OCONNELL, JP .
INDUSTRIAL & ENGINEERING CHEMISTRY PROCESS DESIGN AND DEVELOPMENT, 1975, 14 (03) :209-216