共 25 条
Transport and correlated fluctuations in the nonlinear optical response of excitons
被引:44
作者:

Abramavicius, D.
论文数: 0 引用数: 0
h-index: 0
机构: Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA

Valkunas, L.
论文数: 0 引用数: 0
h-index: 0
机构: Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA

Mukamel, S.
论文数: 0 引用数: 0
h-index: 0
机构: Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA
机构:
[1] Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA
[2] Vilnius State Univ, Fac Phys, Dept Theoret Phys, LT-10222 Vilnius, Lithuania
[3] Inst Phys, LT-02300 Vilnius, Lithuania
来源:
关键词:
D O I:
10.1209/0295-5075/80/17005
中图分类号:
O4 [物理学];
学科分类号:
0702 ;
摘要:
Closed expressions are derived for the femtosecond four-wave mixing of excitons which include slow Gaussian diagonal fluctuations (spectral diffusion) through the cumulant expansion and incoherent exciton transport induced by fast Markovian fluctuations. The interplay of both processes in the two-dimensional photon echo is demonstrated using model calculations for a dimer. Copyright (C) EPLA, 2007.
引用
收藏
页数:6
相关论文
共 25 条
[1]
Two-dimensional spectroscopy of electronic couplings in photosynthesis
[J].
Brixner, T
;
Stenger, J
;
Vaswani, HM
;
Cho, M
;
Blankenship, RE
;
Fleming, GR
.
NATURE,
2005, 434 (7033)
:625-628

Brixner, T
论文数: 0 引用数: 0
h-index: 0
机构: Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA

Stenger, J
论文数: 0 引用数: 0
h-index: 0
机构: Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA

Vaswani, HM
论文数: 0 引用数: 0
h-index: 0
机构: Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA

Cho, M
论文数: 0 引用数: 0
h-index: 0
机构: Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA

Blankenship, RE
论文数: 0 引用数: 0
h-index: 0
机构: Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA

Fleming, GR
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
[2]
Phase-stabilized two-dimensional electronic spectroscopy
[J].
Brixner, T
;
Mancal, T
;
Stiopkin, IV
;
Fleming, GR
.
JOURNAL OF CHEMICAL PHYSICS,
2004, 121 (09)
:4221-4236

Brixner, T
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA

Mancal, T
论文数: 0 引用数: 0
h-index: 0
机构: Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA

Stiopkin, IV
论文数: 0 引用数: 0
h-index: 0
机构: Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA

Fleming, GR
论文数: 0 引用数: 0
h-index: 0
机构: Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
[3]
Collective coordinates for nuclear spectral densities in energy transfer and femtosecond spectroscopy of molecular aggregates
[J].
Chernyak, V
;
Mukamel, S
.
JOURNAL OF CHEMICAL PHYSICS,
1996, 105 (11)
:4565-4583

Chernyak, V
论文数: 0 引用数: 0
h-index: 0
机构: Department of Chemistry, University of Rochester, Rochester

Mukamel, S
论文数: 0 引用数: 0
h-index: 0
机构: Department of Chemistry, University of Rochester, Rochester
[4]
Exciton transport in molecular aggregates probed by time and frequency gated optical spectroscopy
[J].
Chernyak, V
;
Minami, T
;
Mukamel, S
.
JOURNAL OF CHEMICAL PHYSICS,
2000, 112 (18)
:7953-7963

Chernyak, V
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Rochester, Dept Chem, Rochester, NY 14627 USA Univ Rochester, Dept Chem, Rochester, NY 14627 USA

Minami, T
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Rochester, Dept Chem, Rochester, NY 14627 USA Univ Rochester, Dept Chem, Rochester, NY 14627 USA

Mukamel, S
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Rochester, Dept Chem, Rochester, NY 14627 USA Univ Rochester, Dept Chem, Rochester, NY 14627 USA
[5]
PHOTON-ECHOES AND RELATED 4-WAVE-MIXING SPECTROSCOPIES USING PHASE-LOCKED PULSES
[J].
CHO, MH
;
SCHERER, NF
;
FLEMING, GR
;
MUKAMEL, S
.
JOURNAL OF CHEMICAL PHYSICS,
1992, 96 (08)
:5618-5629

CHO, MH
论文数: 0 引用数: 0
h-index: 0
机构: UNIV CHICAGO, JAMES FRANCK INST, CHICAGO, IL 60637 USA

SCHERER, NF
论文数: 0 引用数: 0
h-index: 0
机构: UNIV CHICAGO, JAMES FRANCK INST, CHICAGO, IL 60637 USA

FLEMING, GR
论文数: 0 引用数: 0
h-index: 0
机构: UNIV CHICAGO, JAMES FRANCK INST, CHICAGO, IL 60637 USA

MUKAMEL, S
论文数: 0 引用数: 0
h-index: 0
机构: UNIV CHICAGO, JAMES FRANCK INST, CHICAGO, IL 60637 USA
[6]
Conformational changes during the nanosecond-to-millisecond unfolding of ubiquitin
[J].
Chung, HS
;
Khalil, M
;
Smith, AW
;
Ganim, Z
;
Tokmakoff, A
.
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA,
2005, 102 (03)
:612-617

Chung, HS
论文数: 0 引用数: 0
h-index: 0
机构:
MIT, Dept Chem, Cambridge, MA 02139 USA MIT, Dept Chem, Cambridge, MA 02139 USA

Khalil, M
论文数: 0 引用数: 0
h-index: 0
机构:
MIT, Dept Chem, Cambridge, MA 02139 USA MIT, Dept Chem, Cambridge, MA 02139 USA

Smith, AW
论文数: 0 引用数: 0
h-index: 0
机构:
MIT, Dept Chem, Cambridge, MA 02139 USA MIT, Dept Chem, Cambridge, MA 02139 USA

Ganim, Z
论文数: 0 引用数: 0
h-index: 0
机构:
MIT, Dept Chem, Cambridge, MA 02139 USA MIT, Dept Chem, Cambridge, MA 02139 USA

Tokmakoff, A
论文数: 0 引用数: 0
h-index: 0
机构:
MIT, Dept Chem, Cambridge, MA 02139 USA MIT, Dept Chem, Cambridge, MA 02139 USA
[7]
Correlated vibrational dynamics revealed by two-dimensional infrared spectroscopy -: art. no. 237401
[J].
Demirdöven, N
;
Khalil, M
;
Tokmakoff, A
.
PHYSICAL REVIEW LETTERS,
2002, 89 (23)

Demirdöven, N
论文数: 0 引用数: 0
h-index: 0
机构:
MIT, Dept Chem, Cambridge, MA 02139 USA MIT, Dept Chem, Cambridge, MA 02139 USA

Khalil, M
论文数: 0 引用数: 0
h-index: 0
机构:
MIT, Dept Chem, Cambridge, MA 02139 USA MIT, Dept Chem, Cambridge, MA 02139 USA

Tokmakoff, A
论文数: 0 引用数: 0
h-index: 0
机构:
MIT, Dept Chem, Cambridge, MA 02139 USA MIT, Dept Chem, Cambridge, MA 02139 USA
[8]
Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems
[J].
Engel, Gregory S.
;
Calhoun, Tessa R.
;
Read, Elizabeth L.
;
Ahn, Tae-Kyu
;
Mancal, Tomas
;
Cheng, Yuan-Chung
;
Blankenship, Robert E.
;
Fleming, Graham R.
.
NATURE,
2007, 446 (7137)
:782-786

Engel, Gregory S.
论文数: 0 引用数: 0
h-index: 0
机构: Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA

Calhoun, Tessa R.
论文数: 0 引用数: 0
h-index: 0
机构: Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA

Read, Elizabeth L.
论文数: 0 引用数: 0
h-index: 0
机构: Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA

Ahn, Tae-Kyu
论文数: 0 引用数: 0
h-index: 0
机构: Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA

Mancal, Tomas
论文数: 0 引用数: 0
h-index: 0
机构: Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA

Cheng, Yuan-Chung
论文数: 0 引用数: 0
h-index: 0
机构: Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA

Blankenship, Robert E.
论文数: 0 引用数: 0
h-index: 0
机构: Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA

Fleming, Graham R.
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
[9]
Two-dimensional infrared spectroscopy of isotopomers of an alanine rich α-helix
[J].
Fang, C
;
Wang, J
;
Kim, YS
;
Charnley, AK
;
Barber-Armstrong, W
;
Smith, AB
;
Decatur, SM
;
Hochstrasser, RM
.
JOURNAL OF PHYSICAL CHEMISTRY B,
2004, 108 (29)
:10415-10427

Fang, C
论文数: 0 引用数: 0
h-index: 0
机构: Univ Penn, Dept Chem, Philadelphia, PA 19104 USA

Wang, J
论文数: 0 引用数: 0
h-index: 0
机构: Univ Penn, Dept Chem, Philadelphia, PA 19104 USA

Kim, YS
论文数: 0 引用数: 0
h-index: 0
机构: Univ Penn, Dept Chem, Philadelphia, PA 19104 USA

Charnley, AK
论文数: 0 引用数: 0
h-index: 0
机构: Univ Penn, Dept Chem, Philadelphia, PA 19104 USA

Barber-Armstrong, W
论文数: 0 引用数: 0
h-index: 0
机构: Univ Penn, Dept Chem, Philadelphia, PA 19104 USA

Smith, AB
论文数: 0 引用数: 0
h-index: 0
机构: Univ Penn, Dept Chem, Philadelphia, PA 19104 USA

Decatur, SM
论文数: 0 引用数: 0
h-index: 0
机构: Univ Penn, Dept Chem, Philadelphia, PA 19104 USA

Hochstrasser, RM
论文数: 0 引用数: 0
h-index: 0
机构:
Univ Penn, Dept Chem, Philadelphia, PA 19104 USA Univ Penn, Dept Chem, Philadelphia, PA 19104 USA
[10]
Ultrafast hydrogen-bond dynamics in the infrared spectroscopy of water
[J].
Fecko, CJ
;
Eaves, JD
;
Loparo, JJ
;
Tokmakoff, A
;
Geissler, PL
.
SCIENCE,
2003, 301 (5640)
:1698-1702

Fecko, CJ
论文数: 0 引用数: 0
h-index: 0
机构: MIT, Dept Chem, Cambridge, MA 02139 USA

Eaves, JD
论文数: 0 引用数: 0
h-index: 0
机构: MIT, Dept Chem, Cambridge, MA 02139 USA

Loparo, JJ
论文数: 0 引用数: 0
h-index: 0
机构: MIT, Dept Chem, Cambridge, MA 02139 USA

Tokmakoff, A
论文数: 0 引用数: 0
h-index: 0
机构:
MIT, Dept Chem, Cambridge, MA 02139 USA MIT, Dept Chem, Cambridge, MA 02139 USA

Geissler, PL
论文数: 0 引用数: 0
h-index: 0
机构: MIT, Dept Chem, Cambridge, MA 02139 USA