Pulse-stacked cavity ring-down spectroscopy

被引:38
作者
Crosson, ER [1 ]
Haar, P
Marcus, GA
Schwettman, HA
Paldus, BA
Spence, TG
Zare, RN
机构
[1] Stanford Univ, Stanford FEL Ctr, Dept Phys, Stanford, CA 94305 USA
[2] Stanford Univ, Dept Chem, Stanford, CA 94305 USA
关键词
D O I
10.1063/1.1149533
中图分类号
TH7 [仪器、仪表];
学科分类号
0804 ; 080401 ; 081102 ;
摘要
Pulse stacking, or synchronous pumping, is a novel approach that offers important advantages in cavity ring-down spectroscopy. Using an ultrashort pulse, high repetition rate laser source we have shown that it is possible to resonantly stack pulses in a high finesse cavity, significantly enhancing the decay wave forms obtained when the laser source is abruptly terminated. We have achieved signal-to-noise ratio improvements of several orders of magnitude compared to single pulse injection systems, demonstrating a sensitivity of 2 x 10(-9) cm(-1) at 5.38 mu m. (C) 1999 American Institute of Physics. [S0034-6748(99)04801-7].
引用
收藏
页码:4 / 10
页数:7
相关论文
共 24 条
[1]   A Fourier transform cavity ring down spectrometer [J].
Engeln, R ;
Meijer, G .
REVIEW OF SCIENTIFIC INSTRUMENTS, 1996, 67 (08) :2708-2713
[2]   Phase shift cavity ring down absorption spectroscopy [J].
Engeln, R ;
von Helden, G ;
Berden, G ;
Meijer, G .
CHEMICAL PHYSICS LETTERS, 1996, 262 (1-2) :105-109
[3]   Distributed feedback quantum cascade lasers [J].
Faist, J ;
Gmachl, C ;
Capasso, F ;
Sirtori, C ;
Sivco, DL ;
Baillargeon, JN ;
Cho, AY .
APPLIED PHYSICS LETTERS, 1997, 70 (20) :2670-2672
[4]   Pulse-stacking technique for enhanced performance of a solid-state laser pumped by a high-pulse-rate source [J].
French, SE ;
Brown, DJW ;
Knowles, DS ;
Piper, JA .
APPLIED OPTICS, 1998, 37 (03) :536-539
[5]   PULSE STACKING IN THE SCA/FEL EXTERNAL-CAVITY [J].
HAAR, P ;
SCHWETTMAN, HA ;
SMITH, TI .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 1995, 358 (1-3) :319-322
[6]  
HAAR P, 1994, NUCL INSTRUM METH A, V358, pABS40
[7]  
HAAR P, 1992, NUCL INSTRUM METH A, V331, P621
[8]   Response of a ring-down cavity to an arbitrary excitation [J].
Hodges, JT ;
Looney, JP ;
vanZee, RD .
JOURNAL OF CHEMICAL PHYSICS, 1996, 105 (23) :10278-10288
[9]   Laser bandwidth effects in quantitative cavity ring-down spectroscopy [J].
Hodges, JT ;
Looney, JP ;
vanZee, RD .
APPLIED OPTICS, 1996, 35 (21) :4112-4116
[10]  
KALASHNIKOV VL, 1993, ZHPS, V58, P312