Determination of 241Am in sediments by isotope dilution high resolution inductively coupled plasma mass spectrometry (ID HR ICP-MS)

被引:29
作者
Agarande, M [1 ]
Benzoubir, S [1 ]
Bouisset, P [1 ]
Calmet, D [1 ]
机构
[1] Inst Nucl Safety & Protect, Environm Radioact Measurement Lab, F-91400 Orsay, France
关键词
americium; sediments; ICP-MS;
D O I
10.1016/S0969-8043(01)00045-8
中图分类号
O61 [无机化学];
学科分类号
070301 ; 081704 ;
摘要
Trace levels (pg kg(-1)) of Am-241 in sediments were determined by isotope dilution high resolution inductively coupled plasma mass spectrometry (1D HR ICP-MS) using a microconcentric nebulizer. Am-241 was isolated from major elements like Ca and Fe by different selective precipitations. In Further steps, Am was first separated from other transuranic elements and purified by anion exchange and extraction chromatography prior to the mass spectrometric measurements. The ID HR ICP-MS results are compared with isotope dilution alpha spectrometry. (C) 2001 Elsevier Science Ltd. All rights reserved.
引用
收藏
页码:161 / 165
页数:5
相关论文
共 13 条
[1]  
Crain JS, 1996, SPECTROSCOPY-US, V11, P30
[2]  
DEBIEVRE P, 1978, ADV MASS SPECTROM, V7, P395
[3]   PRECISION MASS SPECTROMETRIC ISOTOPE DILUTION ANALYSIS [J].
DEBIEVRE, PJ ;
DEBUS, GH .
NUCLEAR INSTRUMENTS & METHODS, 1965, 32 (02) :224-&
[4]   METHOD FOR ION-EXCHANGE SEPARATION OF LOW-LEVELS OF AMERICIUM IN ENVIRONMENTAL MATERIALS [J].
HOLM, E ;
BALLESTRA, S ;
FUKAI, R .
TALANTA, 1979, 26 (09) :791-794
[5]   SEPARATION AND PRECONCENTRATION OF ACTINIDES FROM ACIDIC MEDIA BY EXTRACTION CHROMATOGRAPHY [J].
HORWITZ, EP ;
CHIARIZIA, R ;
DIETZ, ML ;
DIAMOND, H .
ANALYTICA CHIMICA ACTA, 1993, 281 (02) :361-372
[6]   APPLICATION OF A HIGH-RESOLUTION INDUCTIVELY COUPLED PLASMA MASS-SPECTROMETER TO THE MEASUREMENT OF LONG-LIVED RADIONUCLIDES [J].
KIM, CK ;
SEKI, R ;
MORITA, S ;
YAMASAKI, S ;
TSUMURA, A ;
TAKAKU, Y ;
IGARASHI, Y ;
YAMAMOTO, M .
JOURNAL OF ANALYTICAL ATOMIC SPECTROMETRY, 1991, 6 (03) :205-209
[7]  
KORKISCH J, 1989, HDB ION EXCHANGE RES, V2, P137
[8]   Determination of 226Ra in mineral waters by high-resolution inductively coupled plasma mass spectrometry after sample preparation by cation exchange [J].
Park, CJ ;
Oh, PJ ;
Kim, HY ;
Lee, DS .
JOURNAL OF ANALYTICAL ATOMIC SPECTROMETRY, 1999, 14 (02) :223-227
[9]   ISOTOPE-DILUTION ALPHA-SPECTROMETRY FOR THE DETERMINATION OF PLUTONIUM CONCENTRATION IN IRRADIATED FUEL DISSOLVER SOLUTION - IDAS AND R-IDAS [J].
RAMANIAH, MV ;
JAIN, HC ;
AGGARWAL, SK ;
CHITAMBAR, SA ;
KAVIMANDAN, VD ;
ALMAULA, AI ;
SHAH, PM ;
PARAB, AR ;
SANT, VL .
NUCLEAR TECHNOLOGY, 1980, 49 (01) :121-128
[10]   High resolution inductively coupled plasma mass spectrometry for the trace determination of plutonium isotopes and isotope ratios in environmental samples [J].
Stürup, S ;
Dahlgaard, H ;
Nielsen, SC .
JOURNAL OF ANALYTICAL ATOMIC SPECTROMETRY, 1998, 13 (12) :1321-1326