Ultrafast energy-transfer dynamics in a blend of electroluminescent conjugated polymers

被引:36
作者
Cerullo, G [1 ]
Nisoli, M
Stagira, S
De Silvestri, S
Lanzani, G
Graupner, W
List, E
Leising, G
机构
[1] Politecn Milan, CEQSE,CNR, Ist Nazl Fis Mat, Dipartimento Fis, I-20133 Milan, Italy
[2] Univ Sassari, Inst Matemat & Fis, I-07100 Sassari, Italy
[3] Graz Tech Univ, Inst Festkorperphys, A-8010 Graz, Austria
关键词
D O I
10.1016/S0009-2614(98)00337-6
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Femtosecond pump-probe spectroscopy was applied to a guest-host system of conjugated polymers, the blue-emitting poly(para-phenylene) (m-LPPP) and the red-emitting poly(perylene-co-diethynylbenzene) (PPDB). Excitation energy transfer between m-LPPP and PPDB, monitored by the formation of the PPDB photobleaching band at 2.15 eV, takes place on a picosecond timescale. The non-exponential kinetics of the excitation energy transfer and its dependence on the acceptor (PPDB) concentration provide clear evidence for a Forster-type energy transfer. (C) 1998 published by Elsevier Science B.V. All rights reserved.
引用
收藏
页码:561 / 566
页数:6
相关论文
共 21 条
  • [1] Berggren M, 1997, NATURE, V389, P466
  • [2] DYNAMICS OF EXCITATION TRANSFER IN DYE-DOPED PI-CONJUGATED POLYMERS
    BOLIVAR, PH
    WEGMANN, G
    KERSTING, R
    DEUSSEN, M
    LEMMER, U
    MAHRT, RF
    BASSLER, H
    GOBEL, EO
    KURZ, H
    [J]. CHEMICAL PHYSICS LETTERS, 1995, 245 (06) : 534 - 538
  • [3] VISIBLE-LIGHT EMISSION FROM SEMICONDUCTING POLYMER DIODES
    BRAUN, D
    HEEGER, AJ
    [J]. APPLIED PHYSICS LETTERS, 1991, 58 (18) : 1982 - 1984
  • [4] LIGHT-EMITTING-DIODES BASED ON CONJUGATED POLYMERS
    BURROUGHES, JH
    BRADLEY, DDC
    BROWN, AR
    MARKS, RN
    MACKAY, K
    FRIEND, RH
    BURN, PL
    HOLMES, AB
    [J]. NATURE, 1990, 347 (6293) : 539 - 541
  • [5] CERULLO G, IN PRESS PHYS REV B
  • [6] Factors influencing stimulated emission from poly(p-phenylenevinylene)
    Denton, GJ
    Tessler, N
    Harrison, NT
    Friend, RH
    [J]. PHYSICAL REVIEW LETTERS, 1997, 78 (04) : 733 - 736
  • [7] *ZWISCHENMOLEKULARE ENERGIEWANDERUNG UND FLUORESZENZ
    FORSTER, T
    [J]. ANNALEN DER PHYSIK, 1948, 2 (1-2) : 55 - 75
  • [8] Femtosecond relaxation of photoexcitations in a poly(para-phenylene)-type ladder polymer
    Graupner, W
    Leising, G
    Lanzani, G
    Nisoli, M
    DeSilvestri, S
    Scherf, U
    [J]. PHYSICAL REVIEW LETTERS, 1996, 76 (05) : 847 - 850
  • [9] GRAUPNER W, 1997, 43 SOC PLAST ENG, P1449
  • [10] ELECTROLUMINESCENCE OF PURE POLY(N-VINYLCARBAZOLE) AND ITS BLENDS WITH A MULTIBLOCK COPOLYMER
    HU, B
    YANG, Z
    KARASZ, FE
    [J]. JOURNAL OF APPLIED PHYSICS, 1994, 76 (04) : 2419 - 2422