Self-similar chain of metal nanospheres as an efficient nanolens

被引:707
作者
Li, KR [1 ]
Stockman, MI
Bergman, DJ
机构
[1] Georgia State Univ, Dept Phys & Astron, Atlanta, GA 30303 USA
[2] Tel Aviv Univ, Raymond & Beverly Sackler Fac Exact Sci, Sch Phys & Astron, IL-69978 Tel Aviv, Israel
基金
以色列科学基金会;
关键词
D O I
10.1103/PhysRevLett.91.227402
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
As an efficient nanolens, we propose a self-similar linear chain of several metal nanospheres with progressively decreasing sizes and separations. To describe such systems, we develop the multipole spectral expansion method. Optically excited, such a nanolens develops the nanofocus ("hottest spot") in the gap between the smallest nanospheres, where the local fields are enhanced by orders of magnitude due to the multiplicative, cascade effect of its geometry and high Q factor of the surface plasmon resonance. The spectral maximum of the enhancement is in the near-ultraviolet region, shifting toward the red region as the separation between the spheres decreases. The proposed system can be used for nanooptical detection, Raman characterization, nonlinear spectroscopy, nanomanipulation of single molecules or nanoparticles, and other applications.
引用
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页数:4
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