Propensity of molecules to spatially align in intense light fields

被引:26
作者
Banerjee, S [1 ]
Mathur, D [1 ]
Kumar, GR [1 ]
机构
[1] Tata Inst Fundamental Res, Mumbai 400005, India
来源
PHYSICAL REVIEW A | 2001年 / 63卷 / 04期
关键词
D O I
10.1103/PhysRevA.63.045401
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
The propensity of molecules to spatially align along the polarization vector of intense, pulsed light fields is related to readily accessible parameters (molecular polarizability, moment of inertia, peak intensity, and pulse duration of the light). It is possible to predict which molecules can be spatially aligned, and under what circumstances, upon exposure to intense light. Accounting for both enhanced ionization and hyperpolarizability, it is shown that all molecules can be aligned, even those with the smallest static polarizability, when subjected to ultrashort pulses of sufficient intensity.
引用
收藏
页码:1 / 4
页数:4
相关论文
共 18 条
[1]   Dynamic and geometric alignment of CS2 in intense laser fields of picosecond and femtosecond duration [J].
Banerjee, S ;
Kumar, GR ;
Mathur, D .
PHYSICAL REVIEW A, 1999, 60 (05) :R3369-R3372
[2]   Intensity-selective, field-induced dissociative ionization of CS2 by femtosecond-duration light pulses [J].
Banerjee, S ;
Kumar, GR ;
Mathur, D .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1999, 32 (17) :4277-4292
[3]   Multiple ionization of N2 in intense, linearly and circularly polarized light fields [J].
Banerjee, S ;
Kumar, GR ;
Mathur, D .
PHYSICAL REVIEW A, 1999, 60 (01) :R25-R28
[4]   Spatial alignment of gas-phase polyatomic molecules by an intense laser field [J].
Bhardwaj, VR ;
Vijayalakshmi, K ;
Mathur, D .
PHYSICAL REVIEW A, 1997, 56 (03) :2455-2458
[5]   FRAGMENT ANGULAR-DISTRIBUTION IN ONE-COLOR AND 2-COLOR PHOTODISSOCIATION BY STRONG LASER FIELDS [J].
CHARRON, E ;
GIUSTISUZOR, A ;
MIES, FH .
PHYSICAL REVIEW A, 1994, 49 (02) :R641-R644
[6]   MOLECULAR-REORIENTATION DURING DISSOCIATIVE MULTIPHOTON IONIZATION [J].
DIETRICH, P ;
STRICKLAND, DT ;
LABERGE, M ;
CORKUM, PB .
PHYSICAL REVIEW A, 1993, 47 (03) :2305-2311
[7]   Laser-induced alignment dynamics of HCN: Roles of the permanent dipole moment and the polarizability [J].
Dion, CM ;
Keller, A ;
Atabek, O ;
Bandrauk, AD .
PHYSICAL REVIEW A, 1999, 59 (02) :1382-1391
[8]   Disentangling molecular alignment and enhanced ionization in intense laser fields [J].
Ellert, C ;
Corkum, PB .
PHYSICAL REVIEW A, 1999, 59 (05) :R3170-R3173
[9]   FEMTOSECOND DYNAMICS OF MULTIELECTRON DISSOCIATIVE IONIZATION BY USE OF PICOSECOND LASER [J].
FRASINSKI, LJ ;
CODLING, K ;
HATHERLY, P ;
BARR, J ;
ROSS, IN ;
TONER, WT .
PHYSICAL REVIEW LETTERS, 1987, 58 (23) :2424-2427
[10]   ALIGNMENT AND TRAPPING OF MOLECULES IN INTENSE LASER FIELDS [J].
FRIEDRICH, B ;
HERSCHBACH, D .
PHYSICAL REVIEW LETTERS, 1995, 74 (23) :4623-4626