A review of the anthropogenic influence on biogenic secondary organic aerosol

被引:237
作者
Hoyle, C. R. [1 ,2 ]
Boy, M. [3 ]
Donahue, N. M. [4 ]
Fry, J. L. [5 ]
Glasius, M. [6 ]
Guenther, A. [7 ]
Hallar, A. G. [8 ]
Hartz, K. Huff [9 ]
Petters, M. D. [12 ]
Petaja, T. [3 ]
Rosenoern, T. [11 ]
Sullivan, A. P. [10 ]
机构
[1] Swiss Fed Inst Technol, Inst Atmospher & Climate Sci, Zurich, Switzerland
[2] Univ Oslo, Dept Geosci, N-0316 Oslo, Norway
[3] Univ Helsinki, Dept Phys, Helsinki 00048, Finland
[4] Carnegie Mellon Univ, Ctr Atmospher Particle Studies, Pittsburgh, PA 15213 USA
[5] Reed Coll, Dept Chem, Portland, OR 97202 USA
[6] Aarhus Univ, Dept Chem, DK-8000 Aarhus C, Denmark
[7] Natl Ctr Atmospher Res, Boulder, CO 80307 USA
[8] Desert Res Inst, Storm Peak Lab, Steamboat Springs, CO USA
[9] So Illinois Univ, Dept Chem & Biochem, Carbondale, IL 62901 USA
[10] Colorado State Univ, Dept Atmospher Sci, Ft Collins, CO 80523 USA
[11] Harvard Univ, Engn Sci Lab 230, Cambridge, MA 02138 USA
[12] N Carolina State Univ, Raleigh, NC 27695 USA
基金
瑞士国家科学基金会; 美国国家科学基金会;
关键词
CLOUD CONDENSATION NUCLEI; BIOMASS BURNING AEROSOLS; FINE-PARTICLE EMISSIONS; PARTICULATE MATTER; SOURCE APPORTIONMENT; SIZE DISTRIBUTION; GAS-PHASE; CHEMICAL-CHARACTERIZATION; AMBIENT AEROSOL; GLOBAL AEROSOL;
D O I
10.5194/acp-11-321-2011
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Because of the climate and air quality effects of organic aerosol, it is important to quantify the influence of anthropogenic emissions on the aerosol burden, both globally and regionally, and both in terms of mass and number. Methods exist with which the fractions of organic aerosol resulting directly from anthropogenic and biogenic processes can be estimated. However, anthropogenic emissions can also lead to an enhancement in secondary organic aerosol formation from naturally emitted precursors. We term this enhanced biogenic secondary organic aerosol (eBSOA). Here, we review the mechanisms through which such an effect may occur in the atmosphere and describe a work flow via which it may be quantified, using existing measurement techniques. An examination of published data reveals support for the existence of the enhancement effect.
引用
收藏
页码:321 / 343
页数:23
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