An In Situ Source-Template-Interface Reaction Route to 3D Nitrogen-Doped Hierarchical Porous Carbon as Oxygen Reduction Electrocatalyst

被引:29
作者
Chen, Yongfang [1 ,2 ]
Ma, Ruguang [1 ,3 ,4 ]
Zhou, Zhenzhen [1 ,3 ]
Liu, Guanghui [1 ,3 ,4 ]
Zhou, Yao [1 ,3 ]
Liu, Qian [1 ,3 ,4 ]
Kaskel, Stefan [5 ]
Wang, Jiacheng [1 ,3 ,4 ]
机构
[1] Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, Shanghai 200050, Peoples R China
[2] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
[3] Chinese Acad Sci, Shanghai Inst Ceram, Innovat Ctr Inorgan Mat Genom Sci, Shanghai 200050, Peoples R China
[4] Shanghai Inst Mat Genome, Shanghai 200444, Peoples R China
[5] Tech Univ Dresden, Dept Inorgan Chem, D-01069 Dresden, Germany
来源
ADVANCED MATERIALS INTERFACES | 2015年 / 2卷 / 11期
基金
中国国家自然科学基金;
关键词
HIGH-PERFORMANCE ELECTROCATALYSTS; METAL-FREE ELECTROCATALYSTS; EFFICIENT ELECTROCATALYSTS; MESOPOROUS MATERIALS; STRUCTURAL-CHANGE; GRAPHENE OXIDE; CATALYST; SURFACE; IRON; CHEMISTRY;
D O I
10.1002/admi.201500199
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
An in situ source-template-interface reaction route is used for the nanocasting synthesis of 3D N-doped hierarchical carbon monolith (NHPCM) composed of interconnected, branched mesoporous rods, with hierarchical porous silicon oxynitride monolith playing both roles of inorganic solid N source and template. The outstanding structural properties of NHPCM render it an excellent metal-free electrocatalyst for oxygen reduction. © 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
引用
收藏
页数:7
相关论文
共 69 条
[1]   From Metal-Organic Framework to Nitrogen-Decorated Nanoporous Carbons: High CO2 Uptake and Efficient Catalytic Oxygen Reduction [J].
Aijaz, Arshad ;
Fujiwara, Naoko ;
Xu, Qiang .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2014, 136 (19) :6790-6793
[2]  
[Anonymous], 2010, ANGEW CHEM-GER EDIT
[3]  
[Anonymous], 2014, Angew. Chem
[4]  
[Anonymous], 1999, ELECTROCHEMICAL SUPE
[5]   A Nitrogen-Doped Graphene/Carbon Nanotube Nanocomposite with Synergistically Enhanced Electrochemical Activity [J].
Chen, Ping ;
Xiao, Tian-Yuan ;
Qian, Yu-Hong ;
Li, Shan-Shan ;
Yu, Shu-Hong .
ADVANCED MATERIALS, 2013, 25 (23) :3192-3196
[6]   Nitrogen-Doped Carbon Nanocages as Efficient Metal-Free Electrocatalysts for Oxygen Reduction Reaction [J].
Chen, Sheng ;
Bi, Jiyu ;
Zhao, Yu ;
Yang, Lijun ;
Zhang, Chen ;
Ma, Yanwen ;
Wu, Qiang ;
Wang, Xizhang ;
Hu, Zheng .
ADVANCED MATERIALS, 2012, 24 (41) :5593-5597
[7]   Surface chemistry of ordered mesoporous carbons [J].
Darmstadt, H ;
Roy, C ;
Kaliaguine, S ;
Choi, SJ ;
Ryoo, R .
CARBON, 2002, 40 (14) :2673-2683
[8]   Electrocatalyst approaches and challenges for automotive fuel cells [J].
Debe, Mark K. .
NATURE, 2012, 486 (7401) :43-51
[9]   The chemistry of graphene oxide [J].
Dreyer, Daniel R. ;
Park, Sungjin ;
Bielawski, Christopher W. ;
Ruoff, Rodney S. .
CHEMICAL SOCIETY REVIEWS, 2010, 39 (01) :228-240
[10]   Mesoporous hybrid material composed of Mn3O4 nanoparticles on nitrogen-doped graphene for highly efficient oxygen reduction reaction [J].
Duan, Jingjing ;
Zheng, Yao ;
Chen, Sheng ;
Tang, Youhong ;
Jaroniec, Mietek ;
Qiao, Shizhang .
CHEMICAL COMMUNICATIONS, 2013, 49 (70) :7705-7707