Pinch points and Kasteleyn transitions in kagome ice

被引:87
作者
Fennell, T.
Bramwell, S. T.
McMorrow, D. F.
Manuel, P.
Wildes, A. R.
机构
[1] London Ctr Nanotechnol, London WC1H 0AJ, England
[2] UCL, Dept Phys, London WC1E 6BT, England
[3] UCL, Dept Chem, London WC1H 0AJ, England
[4] Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England
[5] Inst Max Von Laue Paul Langevin, F-38042 Grenoble 9, France
基金
英国工程与自然科学研究理事会;
关键词
D O I
10.1038/nphys632
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Complex disordered states-from liquids and glasses to exotic quantum matter-are ubiquitous in nature. Their key properties include finite entropy, power-law correlations and emergent organizing principles. In spin ice, spin correlations are determined by the 'ice rules' organizing principle that stabilizes a magnetic state with the same zero-point entropy as water ice. The entropy can be manipulated with great precision by an applied magnetic field: when directed along the three-fold crystallographic axis, the field produces a state of finite entropy, known as kagome ice. Here, we investigate the spin-ice material Ho2Ti2O7 by tilting the magnetic field slightly away from that axis. We thus realize a classic statistical system named after Kasteleyn, in which the entropy of a critical phase can be continuously tuned. Our neutron scattering experiments reveal how this process occurs at a microscopic level.
引用
收藏
页码:566 / 572
页数:7
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