High throughput experimentation for the synthesis of new crystalline microporous solids

被引:38
作者
Newsam, JM
Bein, T
Klein, J
Maier, WF
Stichert, W
机构
[1] Hte Co, Hte N Amer, San Diego, CA 92121 USA
[2] Univ Munich, Dept Chem, D-81377 Munich, Germany
[3] Hte Aktiengesellsch, D-69123 Heidelberg, Germany
[4] Max Planck Inst Kohlenforsch, D-45470 Mulheim, Germany
关键词
high throughput experimentation; zeolite synthesis; structure design; multiclave design; combinatorial chemistry;
D O I
10.1016/S1387-1811(01)00352-3
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
Based on a small number of early experimental results, it can be anticipated that high throughput experimentation (HTE) will play a significant role in the discovery of new zeolites and related materials. The four prime stages in the HTE approach are introduced, in the specific context of work on zeolite synthesis. Key experimental and computational issues are detailed and illustrated by recent literature results. Bottlenecks to achieving the throughput estimated as necessary for a planned level of productivity in new materials discovery are discussed. (C) 2001 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:355 / 365
页数:11
相关论文
共 42 条
[1]  
Akporiaye DE, 1998, ANGEW CHEM INT EDIT, V37, P609, DOI 10.1002/(SICI)1521-3773(19980316)37:5<609::AID-ANIE609>3.0.CO
[2]  
2-X
[3]  
Bein T, 1999, ANGEW CHEM INT EDIT, V38, P323, DOI 10.1002/(SICI)1521-3773(19990201)38:3<323::AID-ANIE323>3.0.CO
[4]  
2-4
[5]  
Box G.E., 1978, STAT EXPT
[6]  
CHAIKEN IM, 1996, ACS S SERIES
[7]  
Choi K, 1999, ANGEW CHEM INT EDIT, V38, P2891, DOI 10.1002/(SICI)1521-3773(19991004)38:19<2891::AID-ANIE2891>3.0.CO
[8]  
2-X
[9]  
Cong PJ, 1999, ANGEW CHEM INT EDIT, V38, P484, DOI 10.1002/(SICI)1521-3773(19990215)38:4<483::AID-ANIE483>3.0.CO
[10]  
2-#